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@ARTICLE{Paulus:862435,
      author       = {Paulus, M. C. and Paulus, A. and Schleker, Peter Philipp
                      Maria and Jakes, P. and Eichel, R.-A. and Heitjans, P. and
                      Granwehr, J.},
      title        = {{E}xperimental evidence for the relaxation coupling of all
                      longitudinal 7{L}i magnetization orders in the superionic
                      conductor {L}i10{G}e{P}2{S}12},
      journal      = {Journal of magnetic resonance},
      volume       = {303},
      issn         = {1090-7807},
      address      = {Amsterdam [u.a.]},
      publisher    = {Elsevier},
      reportid     = {FZJ-2019-02751},
      pages        = {57 - 66},
      year         = {2019},
      abstract     = {This contribution addresses the experimental proof of the
                      relaxation coupling of the 7Li (I = 3/2) longitudinal
                      magnetization orders in the solid-state electrolyte
                      Li10GeP2S12 (LGPS). This effect was theoretically described
                      by Korb and Petit in 1988 but has not yet been shown
                      experimentally. In a 2D-T1/spin-alignment echo (SAE)
                      experiment, the inverse Laplace transformation of the
                      spectral component over two time dimensions revealed the
                      asymmetric course of the spin-lattice relaxation following
                      from the coupling of all longitudinal orders. These
                      observations were supported by Multi-quantum-filter
                      experiments and by simulations of the 2D-T1/SAE experiment
                      with a lithium spin system. Since the asymmetric relaxation
                      effects are directly dependent on the velocities and degrees
                      of freedom of ion motion they could be used especially in
                      fast Li-ion conductors as a separation tool for environments
                      with different mobility processes.},
      cin          = {IEK-9 / IEK-12},
      ddc          = {530},
      cid          = {I:(DE-Juel1)IEK-9-20110218 / I:(DE-Juel1)IEK-12-20141217},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:31004985},
      UT           = {WOS:000468146800007},
      doi          = {10.1016/j.jmr.2019.04.006},
      url          = {https://juser.fz-juelich.de/record/862435},
}