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| 001 | 862435 | ||
| 005 | 20240712113050.0 | ||
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| 100 | 1 | _ | |a Paulus, M. C. |0 P:(DE-Juel1)165914 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Experimental evidence for the relaxation coupling of all longitudinal 7Li magnetization orders in the superionic conductor Li10GeP2S12 |
| 260 | _ | _ | |a Amsterdam [u.a.] |c 2019 |b Elsevier |
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| 520 | _ | _ | |a This contribution addresses the experimental proof of the relaxation coupling of the 7Li (I = 3/2) longitudinal magnetization orders in the solid-state electrolyte Li10GeP2S12 (LGPS). This effect was theoretically described by Korb and Petit in 1988 but has not yet been shown experimentally. In a 2D-T1/spin-alignment echo (SAE) experiment, the inverse Laplace transformation of the spectral component over two time dimensions revealed the asymmetric course of the spin-lattice relaxation following from the coupling of all longitudinal orders. These observations were supported by Multi-quantum-filter experiments and by simulations of the 2D-T1/SAE experiment with a lithium spin system. Since the asymmetric relaxation effects are directly dependent on the velocities and degrees of freedom of ion motion they could be used especially in fast Li-ion conductors as a separation tool for environments with different mobility processes. |
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| 773 | _ | _ | |a 10.1016/j.jmr.2019.04.006 |g Vol. 303, p. 57 - 66 |0 PERI:(DE-600)1469665-4 |p 57 - 66 |t Journal of magnetic resonance |v 303 |y 2019 |x 1090-7807 |
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