000862494 001__ 862494
000862494 005__ 20240712084555.0
000862494 0247_ $$2doi$$a10.1515/ract-2018-3089
000862494 0247_ $$2Handle$$a2128/23429
000862494 0247_ $$2WOS$$aWOS:000489293000008
000862494 037__ $$aFZJ-2019-02800
000862494 041__ $$aEnglish
000862494 082__ $$a610
000862494 1001_ $$0P:(DE-HGF)0$$aMalmbeck, Rikard$$b0
000862494 245__ $$aHomogenous Recycling of Transuranium Elements from Irradiated Fast Reactor Fuel by the EURO-GANEX Solvent Extraction Process
000862494 260__ $$aBerlin$$b˜Deœ Gruyter$$c2019
000862494 3367_ $$2DRIVER$$aarticle
000862494 3367_ $$2DataCite$$aOutput Types/Journal article
000862494 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1574344035_25087
000862494 3367_ $$2BibTeX$$aARTICLE
000862494 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000862494 3367_ $$00$$2EndNote$$aJournal Article
000862494 520__ $$aThe EURO-GANEX process was developed forco-separating transuranium elements from irradiatednuclear fuels. A hot flow-sheet trial was performed in acounter-current centrifugal contactor setup, using a genuinehigh active feed solution. Irradiated mixed (carbide,nitride) U80Pu20 fast reactor fuel containing 20 % Pu wasthermally treated to oxidise it to the oxide form which wasthen dissolved in HNO3. From this solution uranium wasseparated to >99.9 % in a primary solvent extraction cycleusing 1.0 mol/L DEHiBA (N,N-di(2-ethylhexyl)isobutyramidein TPH (hydrogenated tetrapropene) as the organicphase. The raffinate solution from this process, containing10 g/L Pu, was further processed in a second cycle of solventextraction. In this EURO-GANEX flow-sheet, TRU andfission product lanthanides were firstly co-extracted intoa solvent composed of 0.2 mol/L TODGA (N,N,N′,N′-tetran-octyl diglycolamide) and 0.5 mol/L DMDOHEMA (N,N′-dimethyl-N,N′-dioctyl-2-(2-hexyloxy-ethyl) malonamide)dissolved in Exxsol D80, separating them from most otherfission and corrosion products. Subsequently, the TRUwere selectively stripped from the collected loaded solventusing a solution containing 0.055 mol/L SO3-Ph-BTP(2,6-bis(5,6-di(3-sulphophenyl)-1,2,4-triazin-3-yl)pyridinetetrasodium salt) and 1 mol/L AHA (acetohydroxamicacid) in 0.5 mol/L HNO3; lanthanides were finally strippedusing 0.01 mol/L HNO3. Approximately 99.9 % of the TRUand less than 0.1 % of the lanthanides were found in theproduct solution, which also contained the major fractionsof Zr and Mo.
000862494 536__ $$0G:(DE-HGF)POF3-161$$a161 - Nuclear Waste Management (POF3-161)$$cPOF3-161$$fPOF III$$x0
000862494 536__ $$0G:(EU-Grant)211267$$aACSEPT - Actinide reCycling by SEParation and Transmutation (211267)$$c211267$$fFP7-Fission-2007$$x1
000862494 536__ $$0G:(EU-Grant)323282$$aSACSESS - Safety of ACtinide Separation proceSSes (323282)$$c323282$$fFP7-Fission-2012$$x2
000862494 536__ $$0G:(EU-Grant)755171$$aGENIORS - GEN IV Integrated Oxide fuels recycling strategies (755171)$$c755171$$fNFRP-2016-2017-1$$x3
000862494 7001_ $$0P:(DE-HGF)0$$aMugnusson, Daniel$$b1
000862494 7001_ $$0P:(DE-HGF)0$$aBourg, Stéphane$$b2
000862494 7001_ $$0P:(DE-HGF)0$$aCarrott, Michael$$b3
000862494 7001_ $$0P:(DE-HGF)0$$aGeist, Andreas$$b4$$eCorresponding author
000862494 7001_ $$0P:(DE-HGF)0$$aHérès, Xavier$$b5
000862494 7001_ $$0P:(DE-HGF)0$$aMiguirditchian, Manuel$$b6
000862494 7001_ $$0P:(DE-Juel1)130383$$aModolo, Giuseppe$$b7$$ufzj
000862494 7001_ $$0P:(DE-HGF)0$$aMüllich, Udo$$b8
000862494 7001_ $$0P:(DE-HGF)0$$aMiguirditchian, $$b9
000862494 7001_ $$0P:(DE-HGF)0$$aTaylor, Robin$$b10
000862494 7001_ $$0P:(DE-Juel1)130438$$aWilden, Andreas$$b11$$ufzj
000862494 773__ $$0PERI:(DE-600)2039575-9$$a10.1515/ract-2018-3089$$n9-11$$p917-929$$tRadiochimica acta$$v107$$x0033-8230$$y2019
000862494 8564_ $$uhttps://juser.fz-juelich.de/record/862494/files/%5BRadiochimica%20Acta%5D%20Homogenous%20recycling%20of%20transuranium%20elements%20from%20irradiated%20fast%20reactor%20fuel%20by%20the%20EURO-GANEX%20solvent%20extraction%20process.pdf$$yRestricted
000862494 8564_ $$uhttps://juser.fz-juelich.de/record/862494/files/Accepted%20Manuscript.pdf$$yPublished on 2019-05-27. Available in OpenAccess from 2020-05-27.
000862494 8564_ $$uhttps://juser.fz-juelich.de/record/862494/files/Accepted%20Manuscript.pdf?subformat=pdfa$$xpdfa$$yPublished on 2019-05-27. Available in OpenAccess from 2020-05-27.
000862494 909CO $$ooai:juser.fz-juelich.de:862494$$pdnbdelivery$$pec_fundedresources$$pVDB$$pdriver$$popen_access$$popenaire
000862494 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130383$$aForschungszentrum Jülich$$b7$$kFZJ
000862494 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130438$$aForschungszentrum Jülich$$b11$$kFZJ
000862494 9131_ $$0G:(DE-HGF)POF3-161$$1G:(DE-HGF)POF3-160$$2G:(DE-HGF)POF3-100$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$aDE-HGF$$bEnergie$$lNukleare Entsorgung und Sicherheit sowie Strahlenforschung$$vNuclear Waste Management$$x0
000862494 9141_ $$y2019
000862494 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS
000862494 915__ $$0StatID:(DE-HGF)0530$$2StatID$$aEmbargoed OpenAccess
000862494 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bRADIOCHIM ACTA : 2017
000862494 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection
000862494 915__ $$0StatID:(DE-HGF)0110$$2StatID$$aWoS$$bScience Citation Index
000862494 915__ $$0StatID:(DE-HGF)0111$$2StatID$$aWoS$$bScience Citation Index Expanded
000862494 915__ $$0StatID:(DE-HGF)9900$$2StatID$$aIF < 5
000862494 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences
000862494 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline
000862494 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bClarivate Analytics Master Journal List
000862494 920__ $$lyes
000862494 9201_ $$0I:(DE-Juel1)IEK-6-20101013$$kIEK-6$$lNukleare Entsorgung und Reaktorsicherheit$$x0
000862494 9801_ $$aFullTexts
000862494 980__ $$ajournal
000862494 980__ $$aVDB
000862494 980__ $$aUNRESTRICTED
000862494 980__ $$aI:(DE-Juel1)IEK-6-20101013
000862494 981__ $$aI:(DE-Juel1)IFN-2-20101013