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024 7 _ |a 10.1103/PhysRevB.99.144420
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024 7 _ |a 2469-9950
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037 _ _ |a FZJ-2019-02815
082 _ _ |a 530
100 1 _ |a Xu, J.
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245 _ _ |a Anisotropic exchange Hamiltonian, magnetic phase diagram, and domain inversion of Nd2Zr2O7
260 _ _ |a Woodbury, NY
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520 _ _ |a We present thermodynamic and neutron-scattering measurements on the quantum spin ice candidate Nd2Zr2O7. The parametrization of the anisotropic exchange Hamiltonian is refined based on high-energy-resolution inelastic neutron-scattering data together with thermodynamic data using linear spin-wave theory and numerical linked-cluster expansion. Magnetic phase diagrams are calculated using classical Monte Carlo simulations with fields along [100], [110], and [111] crystallographic directions which agree qualitatively with the experiment. Large hysteresis and irreversibility for [111] is reproduced and the microscopic mechanism is revealed by mean-field calculations to be the existence of metastable states and domain inversion. Our results shed light on the explanations of the recently observed dynamical kagome ice in Nd2Zr2O7 in [111] fields.
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542 _ _ |i 2019-04-23
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542 _ _ |i 2020-04-22
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700 1 _ |a Benton, Owen
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700 1 _ |a Anand, V. K.
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700 1 _ |a Islam, A. T. M. N.
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700 1 _ |a Guidi, T.
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700 1 _ |a Ehlers, G.
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700 1 _ |a Gegenwart, P.
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773 _ _ |a 10.1103/PhysRevB.99.144420
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