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@ARTICLE{Li:863003,
      author       = {Li, Dongjiang and Li, Hu and Danilov, Dmitri and Gao, Lu
                      and Chen, Xiaoxuan and Zhang, Zhongru and Zhou, Jiang and
                      Eichel, Rüdiger-A. and Yang, Yong and Notten, Peter H. L.},
      title        = {{D}egradation mechanisms of
                      {C}6/{L}i{N}i0.5{M}n0.3{C}o0.2{O}2 {L}i-ion batteries
                      unraveled by non-destructive and post-mortem methods},
      journal      = {Journal of power sources},
      volume       = {416},
      issn         = {0378-7753},
      address      = {New York, NY [u.a.]},
      publisher    = {Elsevier},
      reportid     = {FZJ-2019-03150},
      pages        = {163 - 174},
      year         = {2019},
      abstract     = {The ageing mechanisms of C6/LiNi0.5Mn0.3Co0.2O2 batteries
                      at various discharging currents and temperatures have
                      systematically been investigated with electrochemical and
                      post-mortem analyses. The irreversible capacity losses () at
                      various ageing conditions are calculated on the basis of
                      regularly determined electromotive force (EMF) curves. Two
                      stages can be distinguished for the degradation of the
                      storage capacity at 30 °C. The first stage includes SEI
                      formation, cathode dissolution, etc. The second stage is
                      related to battery polarization. The various degradation
                      mechanisms of the individual electrodes have been
                      distinguished by vs and vs plots. The
                      Solid-Electrolyte-Interface (SEI) formation as well as the
                      electrode degradation has been experimentally confirmed by
                      XPS analyses. Both Ni and Mn elements are detected at the
                      anode while Co is absent, indicating that the bonding of Co
                      atoms is more robust in the cathode host structure. A
                      Cathode-Electrolyte-Interface (CEI) layer is also detected
                      at the cathode surface. The composition of the CEI layer
                      includes Li salts, such as LiF, LiCOOR, as well as
                      transition metal compounds like NiF2. Cathode dissolution is
                      considered to be responsible for both the NiF2 detected at
                      the cathode and Ni at the anode.},
      cin          = {IEK-9 / IEK-5},
      ddc          = {620},
      cid          = {I:(DE-Juel1)IEK-9-20110218 / I:(DE-Juel1)IEK-5-20101013},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000459839100021},
      doi          = {10.1016/j.jpowsour.2019.01.083},
      url          = {https://juser.fz-juelich.de/record/863003},
}