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| Home > Publications database > Electrochemical Performance of All-Solid-State Sodium-Ion Model Cells with Crystalline Na x CoO 2 Thin-Film Cathodes > print |
| 001 | 863231 | ||
| 005 | 20240711085706.0 | ||
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| 100 | 1 | _ | |a Kehne, P. |0 0000-0002-2760-8337 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Electrochemical Performance of All-Solid-State Sodium-Ion Model Cells with Crystalline Na x CoO 2 Thin-Film Cathodes |
| 260 | _ | _ | |a Pennington, NJ |c 2019 |b Electrochemical Soc. |
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| 520 | _ | _ | |a A common way to improve the electrochemical performance of the NaxCoO2 thin-film cathodes is to increase their crystallinity. Here we present our study of the electrochemical performance of all-solid-state sodium ion batteries with NaxCoO2 thin-film cathodes having two different degrees of crystallinity tuned by their post-deposition annealing at 700°C. The NaxCoO2 cathode thin-films were grown by pulsed laser deposition onto a bulk Na3.4Sc0.4Zr1.6(SiO4)2(PO4) (Nasicon) solid electrolyte substrates and assembled with sodium metal into a Swagelok battery cells. Cells with the low-crystalline NaxCoO2 cathodes show discharge capacities of up to 124 mAh g−1 over 800 charge/discharged cycles. However, cells with highly crystalline NaxCoO2 cathodes revealed a significant capacity loss down to 9 mAh g−1 and a pronounced increase of the overpotential from 100 to 890 mV during the 200 cycles. The observed loss in capacity can be attributed to a strong increase of the interface resistance between the highly crystalline annealed NaxCoO2 films and Nasicon during cycling. |
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| 773 | _ | _ | |a 10.1149/2.0491903jes |g Vol. 166, no. 3, p. A5328 - A5332 |0 PERI:(DE-600)2002179-3 |n 3 |p A5328 - A5332 |t Journal of the Electrochemical Society |v 166 |y 2019 |x 1945-7111 |
| 856 | 4 | _ | |y OpenAccess |u https://juser.fz-juelich.de/record/863231/files/JElectrochemSoc_166_2019_A5328_Kehne.pdf |
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