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| 024 | 7 | _ | |a 2050-7496 |2 ISSN |
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| 100 | 1 | _ | |a Ma, Qianli |0 P:(DE-Juel1)129628 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Room temperature demonstration of a sodium superionic conductor with grain conductivity in excess of 0.01 S cm −1 and its primary applications in symmetric battery cells |
| 260 | _ | _ | |a London [u.a.] |c 2019 |b RSC |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a The lack of suitable candidate electrolyte materials for practical application limits the development of all-solid-state Na-ion batteries. Na3+xZr2Si2+xP1−xO12 was the very first series of NASICONs discovered some 40 years ago; however, separation of bulk conductivity from total conductivity at room temperature is still problematic. It has been suggested that the effective Na-ion conductivity is ∼10−4 S cm−1 at room temperature for Na3+xZr2Si2+xP1−xO12 ceramics; however using a solution-assisted solid-state reaction for preparation of Na3+xZr2Si2+xP1−xO12, a total conductivity of 5 × 10−3 S cm−1 was achieved for Na3.4Zr2Si2.4P0.6O12 at 25 °C, higher than the values previously reported for polycrystalline Na-ion conductors. A bulk conductivity of 1.5 × 10−2 S cm−1 was revealed by high frequency impedance spectroscopy (up to 3 GHz) and verified by low temperature impedance spectroscopy (down to −100 °C) for Na3.4Zr2Si2.4P0.6O12 at 25 °C, indicating further the potential of increasing the related total conductivity. A Na/Na3.4Zr2Si2.4P0.6O12/Na symmetric cell showed low interface resistance and high cycling stability at room temperature. A full-ceramic cell was fabricated and tested at 28 °C with good cycling performance. |
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| 700 | 1 | _ | |a Tsai, Chih-Long |0 P:(DE-Juel1)156244 |b 1 |
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| 700 | 1 | _ | |a Tietz, Frank |0 P:(DE-Juel1)129667 |b 4 |
| 700 | 1 | _ | |a Irvine, John T. S. |0 0000-0002-8394-3359 |b 5 |
| 773 | _ | _ | |a 10.1039/C9TA00048H |g Vol. 7, no. 13, p. 7766 - 7776 |0 PERI:(DE-600)2702232-8 |n 13 |p 7766 - 7776 |t Journal of materials chemistry / A Materials for energy and sustainability A |v 7 |y 2019 |x 2050-7496 |
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