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000863296 1001_ $$0P:(DE-HGF)0$$aSchmitt, Martin$$b0$$eCorresponding author
000863296 245__ $$aIndirect chiral magnetic exchange through Dzyaloshinskii–Moriya-enhanced RKKY interactions in manganese oxide chains on Ir(100)
000863296 260__ $$a[London]$$bNature Publishing Group UK$$c2019
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000863296 520__ $$aLocalized electron spins can couple magnetically via the Ruderman–Kittel–Kasuya–Yosida interaction even if their wave functions lack direct overlap. Theory predicts that spin–orbit scattering leads to a Dzyaloshinskii–Moriya type enhancement of this indirect exchange interaction, giving rise to chiral exchange terms. Here we present a combined spin-polarized scanning tunneling microscopy, angle-resolved photoemission, and density functional theory study of MnO2 chains on Ir(100). Whereas we find antiferromagnetic Mn–Mn coupling along the chain, the inter-chain coupling across the non-magnetic Ir substrate turns out to be chiral with a 120° rotation between adjacent MnO2 chains. Calculations reveal that the Dzyaloshinskii–Moriya interaction results in spin spirals with a periodicity in agreement with experiment. Our findings confirm the existence of indirect chiral magnetic exchange, potentially giving rise to exotic phenomena, such as chiral spin-liquid states in spin ice systems or the emergence of new quasiparticles.
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000863296 7001_ $$00000-0002-7771-8737$$aMoras, Paolo$$b1
000863296 7001_ $$0P:(DE-Juel1)130545$$aBihlmayer, Gustav$$b2
000863296 7001_ $$0P:(DE-HGF)0$$aCotsakis, Ryan$$b3
000863296 7001_ $$0P:(DE-HGF)0$$aVogt, Matthias$$b4
000863296 7001_ $$0P:(DE-HGF)0$$aKemmer, Jeannette$$b5
000863296 7001_ $$0P:(DE-Juel1)162104$$aBelabbes, Abderrezak$$b6
000863296 7001_ $$0P:(DE-HGF)0$$aSheverdyaeva, Polina M.$$b7
000863296 7001_ $$0P:(DE-HGF)0$$aKundu, Asish K.$$b8
000863296 7001_ $$0P:(DE-HGF)0$$aCarbone, Carlo$$b9
000863296 7001_ $$0P:(DE-Juel1)130548$$aBlügel, Stefan$$b10
000863296 7001_ $$00000-0001-7514-5560$$aBode, Matthias$$b11
000863296 773__ $$0PERI:(DE-600)2553671-0$$a10.1038/s41467-019-10515-3$$gVol. 10, no. 1, p. 2610$$n1$$p2610$$tNature Communications$$v10$$x2041-1723$$y2019
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