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100 1 _ |a Schmitt, Martin
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245 _ _ |a Indirect chiral magnetic exchange through Dzyaloshinskii–Moriya-enhanced RKKY interactions in manganese oxide chains on Ir(100)
260 _ _ |a [London]
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520 _ _ |a Localized electron spins can couple magnetically via the Ruderman–Kittel–Kasuya–Yosida interaction even if their wave functions lack direct overlap. Theory predicts that spin–orbit scattering leads to a Dzyaloshinskii–Moriya type enhancement of this indirect exchange interaction, giving rise to chiral exchange terms. Here we present a combined spin-polarized scanning tunneling microscopy, angle-resolved photoemission, and density functional theory study of MnO2 chains on Ir(100). Whereas we find antiferromagnetic Mn–Mn coupling along the chain, the inter-chain coupling across the non-magnetic Ir substrate turns out to be chiral with a 120° rotation between adjacent MnO2 chains. Calculations reveal that the Dzyaloshinskii–Moriya interaction results in spin spirals with a periodicity in agreement with experiment. Our findings confirm the existence of indirect chiral magnetic exchange, potentially giving rise to exotic phenomena, such as chiral spin-liquid states in spin ice systems or the emergence of new quasiparticles.
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700 1 _ |a Moras, Paolo
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700 1 _ |a Bihlmayer, Gustav
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700 1 _ |a Cotsakis, Ryan
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700 1 _ |a Vogt, Matthias
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700 1 _ |a Kemmer, Jeannette
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700 1 _ |a Belabbes, Abderrezak
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700 1 _ |a Sheverdyaeva, Polina M.
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700 1 _ |a Kundu, Asish K.
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700 1 _ |a Carbone, Carlo
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700 1 _ |a Blügel, Stefan
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700 1 _ |a Bode, Matthias
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773 _ _ |a 10.1038/s41467-019-10515-3
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