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@ARTICLE{Janssen:863382,
      author       = {Janssen, Pia and Kasnatscheew, Johannes and Streipert,
                      Benjamin and Wendt, Christian and Murmann, Patrick and
                      Ponomarenko, Maksym and Stubbmann-Kazakova, Olesya and
                      Röschenthaler, Gerd-Volker and Winter, Martin and
                      Cekic-Laskovic, Isidora},
      title        = {{F}luorinated {E}lectrolyte {C}ompound as a
                      {B}i-{F}unctional {I}nterphase {A}dditive for {B}oth,
                      {A}nodes and {C}athodes in {L}ithium-{I}on {B}atteries},
      journal      = {Journal of the Electrochemical Society},
      volume       = {165},
      number       = {14},
      issn         = {1945-7111},
      address      = {Pennington, NJ},
      publisher    = {Electrochemical Soc.},
      reportid     = {FZJ-2019-03455},
      pages        = {A3525 - A3530},
      year         = {2018},
      abstract     = {Lithium-bis(hexafluorobutan-2,3-diol)-borate (R1S),
                      synthesized as a novel electrolyte component in lithium-ion
                      battery (LIB) cells, was evaluated and introduced as a
                      bifunctional interphase additive for both, anodes and
                      cathodes with the purpose of improving the cell performance
                      during high voltage operation. For the graphite based anode
                      it was demonstrated, that the additive could diminish the
                      amount of parasitic capacity required for the formation of
                      an effective solid electrolyte interphase (SEI), which could
                      be concluded from improved Coulombic efficiency data. In
                      parallel, improved capacity retention on the cathode
                      attributed to an altered cathode electrolyte interphase
                      (CEI) by the same additive was observed. Contrary to the CEI
                      formed by the benchmark electrolyte formulation, the
                      interphase of the additive containing electrolyte
                      formulation is significantly influenced in an
                      electrochemical manner (oxidation reactions), as derived
                      from potentiodynamic measurements. As a result, the
                      additive-tuned CEI was found smoother and less resistive
                      compared to the additive-free counterpart, which was
                      demonstrated by electrochemical impedance spectroscopy
                      (EIS), X-ray photoelectron spectroscopy (XPS) and scanning
                      electron microscopy (SEM) of the harvested
                      LiNi1/3Co1/3Mn1/3O2 (NMC111) electrodes after
                      charge/discharge cycling. The simultaneous improvement of
                      the interphases on cathode and anode by the additive could
                      finally enhance the overall performance of a NMC111/graphite
                      cell.},
      cin          = {IEK-12},
      ddc          = {660},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000450275800001},
      doi          = {10.1149/2.1221814jes},
      url          = {https://juser.fz-juelich.de/record/863382},
}