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@INPROCEEDINGS{Ma:863620,
author = {Ma, Qianli and Tietz, Frank and Menzler, Norbert H. and
Guillon, Olivier},
title = {{L}a0.97{N}i0.5{C}o0.5{O}3-δ as air electrode material for
solid oxide cells},
reportid = {FZJ-2019-03632},
year = {2019},
abstract = {Based on former research on perovskites in the
quasi-ternary system LaFeO3–LaCoO3–LaNiO3[1],
LaNi0.5Co0.5O3 (LNC) has been chosen as the most promising
air electrode material for solid oxide cells (SOCs) in this
system. In the present study, A-site deficiency of LNC is
discussed and La0.97Ni0.5Co0.5O3 (LNC97) is selected as the
further optimized composition, which has an electronic
conductivity of over 1000 S cm-1 at 800oC [2] .
Compatibility of LNC97 with 8 $mol\%$ Y2O3 stabilized ZrO2
(8YSZ) is analyzed and compared with that of
La0.58Sr0.4Co0.8Fe0.2O3-δ (LSCF) and 8YSZ. According to the
requirements of the air electrode materials with qualified
performance, i.e. 1) high electronic conductivity, 2) high
ionic conductivity, and 3) high catalytic activity for the
oxygen reduction reaction, LNC97 based electrodes are
modified, characterized and optimized by symmetric cell
tests. Degradation of the symmetric cells after 1000 h of
operation is discussed. Mechanisms for explaining the
electrode-processes of LNC97-based electrodes are raised.
Full cells based on optimized LNC97 material were tested
under both fuel cell mode and electrolyzer mode. The
achieved performances are even better than
the-state-of-the-art LSCF based SOCs, indicating a
prospective future for the developed material and the
air-electrode.[1] F. Tietz, I. ArulRaj, Q. Ma, S.Baumann,
A.Mahmoud, R.P.Hermann, J. Solid State Chem. 237 (2016)
183–191.[2] Q. Ma, M. Balaguer, D. Pérez-Coll, L. G. J.
de Haart, J. M. Serra, G. C. Mather, F. Tietz, N. H.
Menzler, O. Guillon. ACS Appl. Energy Mater. 1 (2018)
2784−2792.},
month = {Jun},
date = {2019-06-16},
organization = {The 22nd International Conference on
Solid State Ionics 22nd International
Conference on Solid State Ionics,
PyeongChang (Korea), 16 Jun 2019 - 21
Jun 2019},
subtyp = {After Call},
cin = {IEK-1},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {135 - Fuel Cells (POF3-135) / SOFC - Solid Oxide Fuel Cell
(SOFC-20140602)},
pid = {G:(DE-HGF)POF3-135 / G:(DE-Juel1)SOFC-20140602},
typ = {PUB:(DE-HGF)6},
url = {https://juser.fz-juelich.de/record/863620},
}