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@ARTICLE{Zoller:864084,
      author       = {Zoller, Florian and Luxa, Jan and Bein, Thomas and
                      Fattakhova-Rohlfing, Dina and Bouša, Daniel and Sofer,
                      Zdeněk},
      title        = {{F}lexible freestanding {M}o{S} 2 -based composite paper
                      for energy conversion and storage},
      journal      = {Beilstein journal of nanotechnology},
      volume       = {10},
      issn         = {2190-4286},
      address      = {Frankfurt, M.},
      publisher    = {Beilstein-Institut zur Förderung der Chemischen
                      Wissenschaften},
      reportid     = {FZJ-2019-03991},
      pages        = {1488 - 1496},
      year         = {2019},
      abstract     = {The construction of flexible electrochemical devices for
                      energy storage and generation is of utmost importance in
                      modern society. In this article, we report on the synthesis
                      of flexible MoS2-based composite paper by high-energy shear
                      force milling and simple vacuum filtration. This composite
                      material combines high flexibility, mechanical strength and
                      good chemical stability. Chronopotentiometric
                      charge–discharge measurements were used to determine the
                      capacitance of our paper material. The highest capacitance
                      achieved was 33 mF·cm−2 at a current density of 1
                      mA·cm−2, demonstrating potential application in
                      supercapacitors. We further used the material as a cathode
                      for the hydrogen evolution reaction (HER) with an onset
                      potential of approximately −0.2 V vs RHE. The onset
                      potential was even lower (approximately −0.1 V vs RHE)
                      after treatment with n-butyllithium, suggesting the
                      introduction of new active sites. Finally, a potential use
                      in lithium ion batteries (LIB) was examined. Our material
                      can be used directly without any binder, additive carbon or
                      copper current collector and delivers specific capacity of
                      740 mA·h·g−1 at a current density of 0.1 A·g−1. After
                      40 cycles at this current density the material still reached
                      a capacity retention of $91\%.$ Our findings show that this
                      composite material could find application in electrochemical
                      energy storage and generation devices where high flexibility
                      and mechanical strength are desired.Keywords: flexible
                      composites; hydrogen evolution reaction (HER); lithium ion
                      batteries (LIBs); molybdenum disulfide; nanoarchitectonics;
                      supercapacitors},
      cin          = {IEK-1},
      ddc          = {620},
      cid          = {I:(DE-Juel1)IEK-1-20101013},
      pnm          = {899 - ohne Topic (POF3-899)},
      pid          = {G:(DE-HGF)POF3-899},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000476926400002},
      doi          = {10.3762/bjnano.10.147},
      url          = {https://juser.fz-juelich.de/record/864084},
}