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@ARTICLE{Yan:864390,
author = {Yan, Gang and Yu, Shicheng and Yang, Weiguang and Xiaqiang,
Li and Tempel, Hermann and Kungl, Hans and Eichel,
Rüdiger-A. and Krüger, Manja and Malzbender, Jürgen},
title = {{A}nisotropy of the mechanical properties of
{L}i1·3{A}l0·3{T}i1·7({PO}4)3 solid electrolyte material},
journal = {Journal of power sources},
volume = {437},
issn = {0378-7753},
address = {New York, NY [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2019-04182},
pages = {226940 -},
year = {2019},
abstract = {Solid state lithium ion batteries have high potential for
future energy storage since they promise high energy density
and safety, latter being related to the mechanical
properties of the materials. For example the micro-battery,
being one application of the solid state batteries, requires
a thin solid electrolyte, which renders especially
anisotropic behavior of the materials’ properties
important. In particular, Li1+xAlxTi2-x (PO4)3 (LATP) is a
promising solid electrolyte material that possesses a
rhombohedral crystal structure that might lead to such
anisotropic mechanical properties. In current work a
nanoindentation test is combined with EBSD technique to
correlate elastic modulus and hardness of LATP to the
crystal orientation. Furthermore, calculations based on the
Vlassak-Nix and easy-slip models are adopted to verify the
anisotropic mechanical properties. Overall, the
experimentally derived elastic modulus and hardness of LATP
show similar trends. The experimentally derived indentation
modulus agrees well with the prediction of the Vlassak-Nix
model. The normalization of the experimentally derived
hardness and the hardness ratio from the easy-slip model
reveal comparable trends. This work aids a deepening of the
understanding of the mechanical properties of LATP
electrolyte and provides a basis for further improvement of
the Vlassak-Nix and easy-slip models in the application to
rhombohedral materials.},
cin = {IEK-2 / IEK-9},
ddc = {620},
cid = {I:(DE-Juel1)IEK-2-20101013 / I:(DE-Juel1)IEK-9-20110218},
pnm = {131 - Electrochemical Storage (POF3-131)},
pid = {G:(DE-HGF)POF3-131},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000486355400009},
doi = {10.1016/j.jpowsour.2019.226940},
url = {https://juser.fz-juelich.de/record/864390},
}