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| Hauptseite > Workflowsammlungen > Publikationsgebühren > High-Temperature Co-Electrolysis: A Versatile Method to Sustainably Produce Tailored Syngas Compositions > print |
| Hauptseite > Workflowsammlungen > Publikationsgebühren > High-Temperature Co-Electrolysis: A Versatile Method to Sustainably Produce Tailored Syngas Compositions > print |
| 001 | 864472 | ||
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| 100 | 1 | _ | |a Dittrich, Lucy |0 P:(DE-Juel1)171748 |b 0 |e Corresponding author |
| 245 | _ | _ | |a High-Temperature Co-Electrolysis: A Versatile Method to Sustainably Produce Tailored Syngas Compositions |
| 260 | _ | _ | |a Pennington, NJ |c 2019 |b Electrochemical Soc. |
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| 520 | _ | _ | |a High-temperature co-electrolysis of carbon dioxide and steam is a promising method to produce ‘white’ syngas by making use of renewable energy and carbon dioxide as sustainable feedstock. The technological key advantage is the possibility to tailor syngas compositions over a broad range. This paper presents a systematic investigation of the syngas tailoring process by establishing relationships between feed gas compositions and flow rates to the syngas ratio. A linear dependence between the H2O:CO2 ratio in the feed gas and the H2:CO ratio in the output gas was observed. Furthermore, the syngas ratio remains mostly invariant upon variations in electrochemical potential and fluctuating gas utilizations/flow rates during operation of a co-electrolysis cell. Most importantly, the co-electrolysis performance was demonstrated to operate at high current densities of up to 3.2 A·cm−2 over a broad range of feed gas compositions with faradaic efficiencies of nearly 100%. The possibility to operate co-electrolysis under transient load conditions renders this method particularly suitable in future scenarios of intermittent availability of renewables. The results described here illustrate the versatility of co-electrolysis, which can produce all relevant syngas compositions in a single-step process at constantly high performance. |
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| 773 | _ | _ | |a 10.1149/2.0581913jes |g Vol. 166, no. 13, p. F971 - F975 |0 PERI:(DE-600)2002179-3 |n 13 |p F971 - F975 |t Journal of the Electrochemical Society |v 166 |y 2019 |x 0013-4651 |
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