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@ARTICLE{Wang:864625,
      author       = {Wang, Hongjia and Wang, Yanjie and Guo, Lingju and Zhang,
                      Xuehua and Ribeiro de Oliveira, Caue and He, Tao},
      title        = {{S}olar-{H}eating {B}oosted {C}atalytic {R}eduction of
                      {CO}2 under {F}ull-{S}olar {S}pectrum},
      journal      = {Chinese journal of catalysis},
      volume       = {41},
      number       = {1},
      issn         = {0253-9837},
      address      = {Amsterdam [u.a.]},
      publisher    = {Elsevier},
      reportid     = {FZJ-2019-04330},
      pages        = {131 - 139},
      year         = {2020},
      abstract     = {Catalytic converting CO2 into fuels with the help of solar
                      energy is regarded as ‘dream reaction’, as both energy
                      crisis and environmental issue can be mitigated
                      simultaneously. However, it is still suffering from low
                      efficiency due to narrow solar-spectrum utilization and
                      sluggish heterogeneous reaction kinetics. In this work, we
                      demonstrate that catalytic reduction of CO2 can be achieved
                      over Au nanoparticles (NPs) deposited rutile under full
                      solar-spectrum irradiation, boosted by solar-heating effect.
                      We found that UV and visible light can initiate the
                      reaction, and the heat from IR light and local
                      surface-plasmon resonance relaxation of Au NPs can boost the
                      reaction kinetically. The apparent activation energy is
                      determined experimentally and is used to explain the
                      superior catalytic activity of Au/rutile to rutile in a
                      kinetic way. We also find the photo-thermal synergy in the
                      Au/rutile system. We envision that this work may facilitate
                      understanding the kinetics of CO2 reduction and developing
                      feasible catalytic systems with full solar spectrum
                      utilization for practical artificial photosynthesis.},
      cin          = {IEK-14},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-14-20191129},
      pnm          = {134 - Electrolysis and Hydrogen (POF3-134)},
      pid          = {G:(DE-HGF)POF3-134},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000495145800015},
      doi          = {10.1016/S1872-2067(19)63393-0},
      url          = {https://juser.fz-juelich.de/record/864625},
}