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000865028 1001_ $$0P:(DE-Juel1)6121$$aKotov, Vladislav$$b0$$eCorresponding author
000865028 245__ $$aPlug flow reactor model of the plasma chemical conversion of CO2
000865028 260__ $$aBristol$$bIOP Publ.$$c2019
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000865028 520__ $$aA 1D plug flow model suitable for describing the CO<sub>2</sub> conversion into CO in microwave plasma reactors is proposed. The model is applied together with the Antwerp data set for the CO<sub>2</sub> reaction kinetics to calculate parameter scans for a realistic experimental set up. The energy re-distribution pathways in the model calculations are analyzed. The analysis shows that despite the input power is initially deposited mainly into vibrational states the fast vibrational-translational (VT) transfer leads to dissociation of CO<sub>2</sub> predominantly via the thermal quenching mechanism. Solutions with mitigated VT-losses can be obtained by increasing the specific input power - power per unit volume. In this regime the energy efficiency starts to be constrained by reverse processes.
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000865028 7001_ $$0P:(DE-HGF)0$$aKoelman, Peter$$b1
000865028 773__ $$0PERI:(DE-600)2004012-X$$a10.1088/1361-6595/ab3774$$n9$$p095002$$tPlasma sources science and technology$$v28$$x1361-6595$$y2019
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