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@ARTICLE{Sazonov:865103,
author = {Sazonov, Andrew and Hutanu, Vladimir and Meven, Martin and
Röwer, Karine and Roth, Georg and Lelièvre-Berna, Eddy and
Fuchs, Günther and Zaharko, Oksana and Friese, Karen},
title = {{U}nambiguous determination of the commensurate
antiferromagnetic structure of {H}o{N}i 2 {B} 2 {C} in the
superconducting ground state},
journal = {Physical review / B},
volume = {100},
number = {1},
issn = {2469-9950},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {FZJ-2019-04659},
pages = {014414},
year = {2019},
abstract = {Crystal and magnetic structures of the intermetallic
HoNi2B2C have been investigated using different
single-crystal diffraction techniques at both room and low
temperatures (superconducting phase). Combined refinement of
the neutron and x-ray diffraction data performed at room
temperature shows that the crystal structure of HoNi2B2C is
well described in the tetragonal space group I4/mmm, in
agreement with the literature. The magnetic ordering at low
temperatures is accompanied by a structural phase transition
to the orthorhombic space group Fmmm. However, only
noncharacteristic orbits are occupied in this space group,
and the symmetry reduction is entirely due to a lifting of
the symmetry-induced restrictions on the anisotropic
displacement parameters. Based on magnetic symmetry
analysis, two types of commensurate antiferromagnetic
structures with different magnetic space groups (MSGs) are
found below TN≈5.2 K: MSG PInnm (Ho spins are along the
[100] direction of the parent structure) and MSG CAmca (Ho
spins are along [110] of the parent structure). Both models
agree well with conventional unpolarized neutron diffraction
data at low temperature (2.4 K) with ordered magnetic
moments of 9.16(9) μB/Ho3+ atom. Spherical neutron
polarimetry, on the other hand, allowed us to unambiguously
solve the magnetic structure (MSG CAmca) as well as to
determine the population of two types of 90∘
antiferromagnetic domains (0.45/0.55).},
cin = {JCNS-FRM-II / MLZ / JCNS-2},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 / I:(DE-588b)4597118-3 /
I:(DE-Juel1)JCNS-2-20110106},
pnm = {524 - Controlling Collective States (POF3-524) / 6212 -
Quantum Condensed Matter: Magnetism, Superconductivity
(POF3-621) / 6G15 - FRM II / MLZ (POF3-6G15) / 6G4 - Jülich
Centre for Neutron Research (JCNS) (POF3-623)},
pid = {G:(DE-HGF)POF3-524 / G:(DE-HGF)POF3-6212 /
G:(DE-HGF)POF3-6G15 / G:(DE-HGF)POF3-6G4},
experiment = {EXP:(DE-MLZ)HEIDI-20140101 /
EXP:(DE-MLZ)POLI-HEIDI-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000475496800002},
doi = {10.1103/PhysRevB.100.014414},
url = {https://juser.fz-juelich.de/record/865103},
}