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000865114 1001_ $$00000-0003-1881-2018$$aSteiner, Anja Maria$$b0
000865114 245__ $$aSilver Particles with Rhombicuboctahedral Shape and Effective Isotropic Interactions with Light
000865114 260__ $$aWashington, DC$$bAmerican Chemical Society$$c2019
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000865114 520__ $$aTruly spherical silver nanoparticles are of great importance for fundamental studies including plasmonic applications, but their direct synthesis in aqueous media is not feasible. Using the commonly employed copper-based etching processes, an isotropic plasmonic response can be achieved by etching well-defined silver nanocubes. Whilst spherical-like shape is typically prevailing in such processes, we established that there is a preferential growth toward silver rhombicuboctahedra, which is the thermodynamically most stable product of this synthesis. The rhombicuboctahedral morphology is further evidenced by comprehensive characterization with small-angle X-ray scattering in combination with transmission electron microscopy (TEM) tomography and high-resolution TEM. We also elucidate the complete reaction mechanism based on UV–vis kinetic studies, and the postulated mechanism can also be extended to all copper-based etching processes
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000865114 7001_ $$00000-0003-4013-1892$$aMayer, Martin$$b1
000865114 7001_ $$0P:(DE-HGF)0$$aSchletz, Daniel$$b2
000865114 7001_ $$00000-0001-5000-8578$$aWolf, Daniel$$b3
000865114 7001_ $$0P:(DE-HGF)0$$aFormanek, Petr$$b4
000865114 7001_ $$0P:(DE-HGF)0$$aHübner, René$$b5
000865114 7001_ $$0P:(DE-Juel1)172746$$aDulle, Martin$$b6
000865114 7001_ $$0P:(DE-Juel1)172658$$aFörster, Stephan$$b7
000865114 7001_ $$00000-0002-8852-8752$$aKönig, Tobias A. F.$$b8
000865114 7001_ $$00000-0001-6692-3762$$aFery, Andreas$$b9$$eCorresponding author
000865114 773__ $$0PERI:(DE-600)1500399-1$$a10.1021/acs.chemmater.8b05220$$gVol. 31, no. 8, p. 2822 - 2827$$n8$$p2822 - 2827$$tChemistry of materials$$v31$$x1520-5002$$y2019
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000865114 8564_ $$uhttps://juser.fz-juelich.de/record/865114/files/1910.07764.pdf$$yPublished on 2019-03-18. Available in OpenAccess from 2020-03-18.
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