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@ARTICLE{Steiner:865114,
      author       = {Steiner, Anja Maria and Mayer, Martin and Schletz, Daniel
                      and Wolf, Daniel and Formanek, Petr and Hübner, René and
                      Dulle, Martin and Förster, Stephan and König, Tobias A. F.
                      and Fery, Andreas},
      title        = {{S}ilver {P}articles with {R}hombicuboctahedral {S}hape and
                      {E}ffective {I}sotropic {I}nteractions with {L}ight},
      journal      = {Chemistry of materials},
      volume       = {31},
      number       = {8},
      issn         = {1520-5002},
      address      = {Washington, DC},
      publisher    = {American Chemical Society},
      reportid     = {FZJ-2019-04666},
      pages        = {2822 - 2827},
      year         = {2019},
      abstract     = {Truly spherical silver nanoparticles are of great
                      importance for fundamental studies including plasmonic
                      applications, but their direct synthesis in aqueous media is
                      not feasible. Using the commonly employed copper-based
                      etching processes, an isotropic plasmonic response can be
                      achieved by etching well-defined silver nanocubes. Whilst
                      spherical-like shape is typically prevailing in such
                      processes, we established that there is a preferential
                      growth toward silver rhombicuboctahedra, which is the
                      thermodynamically most stable product of this synthesis. The
                      rhombicuboctahedral morphology is further evidenced by
                      comprehensive characterization with small-angle X-ray
                      scattering in combination with transmission electron
                      microscopy (TEM) tomography and high-resolution TEM. We also
                      elucidate the complete reaction mechanism based on UV–vis
                      kinetic studies, and the postulated mechanism can also be
                      extended to all copper-based etching processes},
      cin          = {ICS-1 / JCNS-1},
      ddc          = {540},
      cid          = {I:(DE-Juel1)ICS-1-20110106 / I:(DE-Juel1)JCNS-1-20110106},
      pnm          = {551 - Functional Macromolecules and Complexes (POF3-551) /
                      6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)
                      / 6215 - Soft Matter, Health and Life Sciences (POF3-621)},
      pid          = {G:(DE-HGF)POF3-551 / G:(DE-HGF)POF3-6G4 /
                      G:(DE-HGF)POF3-6215},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000466053300017},
      doi          = {10.1021/acs.chemmater.8b05220},
      url          = {https://juser.fz-juelich.de/record/865114},
}