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@ARTICLE{Zips:865138,
author = {Zips, Sabine and Grob, Leroy and Rinklin, Philipp and
Terkan, Korkut and Adly, Nouran Yehia and Weiß, Lennart
Jakob Konstantin and Mayer, Dirk and Wolfrum, Bernhard},
title = {{F}ully {P}rinted μ-{N}eedle {E}lectrode {A}rray from
{C}onductive {P}olymer {I}nk for {B}ioelectronic
{A}pplications},
journal = {ACS applied materials $\&$ interfaces},
volume = {11},
number = {36},
issn = {1944-8252},
address = {Washington, DC},
publisher = {Soc.},
reportid = {FZJ-2019-04690},
pages = {32778 - 32786},
year = {2019},
abstract = {Microelectrode arrays (MEAs) are widely used platforms in
bioelectronics to study electrogenic cells. In recent years,
the processing of conductive polymers for the fabrication of
three-dimensional electrode arrays has gained increasing
interest for the development of novel sensor designs. Here,
additive manufacturing techniques are promising tools for
the production of MEAs with three-dimensional electrodes. In
this work, a facile additive manufacturing process for the
fabrication of MEAs that feature needle-like electrode tips,
so-called μ-needles, is presented. To this end, an
aerosol-jet compatible PEDOT:PSS and multiwalled carbon
nanotube composite ink with a conductivity of 323 ± 75 S
m–1 is developed and used in a combined inkjet and
aerosol-jet printing process to produce the μ-needle
electrode features. The μ-needles are fabricated with a
diameter of 10 ± 2 μm and a height of 33 ± 4 μm. They
penetrate an inkjet-printed dielectric layer to a height of
12 ± 3 μm. After successful printing, the electrochemical
properties of the devices are assessed via cyclic
voltammetry and impedance spectroscopy. The μ-needles show
a capacitance of 242 ± 70 nF at a scan rate of 5 mV s–1
and an impedance of 128 ± 22 kΩ at 1 kHz frequency. The
stability of the μ-needle MEAs in aqueous electrolyte is
demonstrated and the devices are used to record
extracellular signals from cardiomyocyte-like HL-1 cells.
This proof-of-principle experiment shows the μ-needle
MEAs’ cell-culture compatibility and functional integrity
to investigate electrophysiological signals from living
cells.},
cin = {ICS-8},
ddc = {600},
cid = {I:(DE-Juel1)ICS-8-20110106},
pnm = {552 - Engineering Cell Function (POF3-552)},
pid = {G:(DE-HGF)POF3-552},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:31424902},
UT = {WOS:000486360500020},
doi = {10.1021/acsami.9b11774},
url = {https://juser.fz-juelich.de/record/865138},
}