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@ARTICLE{Songvilay:865225,
author = {Songvilay, M. and Giles-Donovan, N. and Bari, M. and Ye, Z.
-G. and Minns, J. L. and Green, M. A. and Xu, Guangyong and
Gehring, P. M. and Schmalzl, K. and Ratcliff, W. D. and
Brown, C. and Chernyshov, D. and Van Beek, W. and Cochran,
S. and Stock, C.},
title = {{C}ommon acoustic phonon damping in inorganic and hybrid
lead halide perovskites},
journal = {Physical review materials},
volume = {3},
issn = {2475-9953},
address = {College Park, MD},
publisher = {APS},
reportid = {FZJ-2019-04759},
pages = {093602},
year = {2019},
abstract = {The acoustic phonons in the organic-inorganic lead halide
perovskites have been reported to have anomalously short
lifetimes over a large part of the Brillouin zone. The
resulting shortened mean free paths of the phonons have been
implicated as the origin of the low thermal conductivity. We
apply neutron spectroscopy to show that the same acoustic
phonon energy linewidth broadening occurs in the fully
inorganic CsPbBr$_{3}$ by comparing the results on the
organic-inorganic CH$_{3}$NH$_{3}$PbCl$_{3}$. We investigate
the critical dynamics near the three zone boundaries of the
cubic $Pm\overline{3}m$ Brillouin zone of CsPbBr$_{3}$ and
find energy and momentum broadened dynamics at momentum
points where the Cs-site ($A$-site) motions contribute to
the cross section. Neutron diffraction is used to confirm
that both the Cs and Br sites have unusually large thermal
displacements with an anisotropy that mirrors the low
temperature structural distortions. The presence of an
organic molecule is not necessary to disrupt the low-energy
acoustic phonons at momentum transfers located away from the
zone center in the lead halide perovskites and such damping
may be driven by the large displacements or possibly
disorder on the $A$ site.},
cin = {JCNS-2 / PGI-4 / JARA-FIT / JCNS-ILL},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)PGI-4-20110106 /
$I:(DE-82)080009_20140620$ / I:(DE-Juel1)JCNS-ILL-20110128},
pnm = {144 - Controlling Collective States (POF3-144) / 524 -
Controlling Collective States (POF3-524) / 6212 - Quantum
Condensed Matter: Magnetism, Superconductivity (POF3-621) /
6213 - Materials and Processes for Energy and Transport
Technologies (POF3-621) / 6G4 - Jülich Centre for Neutron
Research (JCNS) (POF3-623)},
pid = {G:(DE-HGF)POF3-144 / G:(DE-HGF)POF3-524 /
G:(DE-HGF)POF3-6212 / G:(DE-HGF)POF3-6213 /
G:(DE-HGF)POF3-6G4},
experiment = {EXP:(DE-Juel1)ILL-IN12-20150421},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000486663700001},
doi = {10.1103/PhysRevMaterials.3.093602},
url = {https://juser.fz-juelich.de/record/865225},
}