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@ARTICLE{Raijmakers:866397,
      author       = {Raijmakers, Luc and Danilov, Dmitri and Eichel, Rüdiger-A.
                      and Notten, Peter H. L.},
      title        = {{A}n advanced all-solid-state {L}i-ion battery model},
      journal      = {Electrochimica acta},
      volume       = {330},
      issn         = {0013-4686},
      address      = {New York, NY [u.a.]},
      publisher    = {Elsevier},
      reportid     = {FZJ-2019-05551},
      pages        = {135147 -},
      year         = {2020},
      abstract     = {A new advanced mathematical model is proposed to accurately
                      simulate the behavior of all-solid-state Li-ion batteries.
                      The model includes charge-transfer kinetics at both
                      electrode/electrolyte interfaces, diffusion and migration of
                      mobile lithium ions in the electrolyte and positive
                      electrode. In addition, electrical double layers are
                      considered, representing the space-charge separation
                      phenomena at both electrode/electrolyte interfaces. The
                      model can be used to simultaneously study the individual
                      overpotential and impedance contributions together with
                      concentration gradients and electric fields across the
                      entire battery stack. Both galvanostatic discharge and
                      impedance simulations have been experimentally validated
                      with respect to 0.7 mAh // thin film, all-solid-state,
                      batteries. The model shows good agreement with galvanostatic
                      discharging, voltage relaxation upon current interruption,
                      and impedance measurements. From the performed AC and DC
                      simulations it can be concluded that the overpotential
                      across the electrolyte is most dominant and is therefore an
                      important rate-limiting factor. In addition, it is found
                      that both ionic and electronic diffusion coefficients in the
                      electrode seriously influence the battery performance. The
                      present model is generally applicable to all-solid-state
                      batteries where combined ionic and electronic transport
                      takes place and allows for optimizing the battery components
                      to increase the effective energy density, which leads to a
                      decreasing demand for materials and costs.},
      cin          = {IEK-9},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-9-20110218},
      pnm          = {135 - Fuel Cells (POF3-135)},
      pid          = {G:(DE-HGF)POF3-135},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000501468400002},
      doi          = {10.1016/j.electacta.2019.135147},
      url          = {https://juser.fz-juelich.de/record/866397},
}