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@ARTICLE{Lewerenz:866894,
author = {Lewerenz, Meinert and Fuchs, Georg and Becker, Lisa and
Sauer, Dirk Uwe},
title = {{I}rreversible calendar aging and quantification of the
reversible capacity loss caused by anode overhang},
journal = {Journal of energy storage},
volume = {18},
issn = {2352-152X},
address = {Amsterdam [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2019-05954},
pages = {149 - 159},
year = {2018},
abstract = {Calendar aging tests are presented quantifying the
reversible capacity loss caused by lithium migration from
the active part to the overhang of the anode. Based on these
tests, capacity loss at five different SOCs with respect to
the anode is evaluated. The remaining capacity shows a
non-linear part in the beginning representing the reversible
capacity loss caused by the overhang. The subsequent linear
part ending after 100–200 days corresponds to the
irreversible capacity loss. By extrapolating the linear part
to t = 0, the lithium lost to the overhang is
measureable for each storage condition. This approach
matches well to theoretical values calculated using a simple
equation. In later stages of the capacity loss curve,
another superposed effect can be observed that decreases
capacity fade. The reason is found in an increasing
homogeneity of lithium distribution that correlates to the
peak height of differential voltage characteristics. In this
publication an increasing homogeneity is associated with a
higher extractable capacity and vice versa. An especially
high increase of homogeneity is observable when a high
voltage difference coincides with pressure change due to
lithium insertion. Finally, the temperature dependency of
the lateral lithium flow is shown for three temperatures at
a fixed storage position.},
cin = {IEK-12 / JARA-ENERGY},
ddc = {333.7},
cid = {I:(DE-Juel1)IEK-12-20141217 / $I:(DE-82)080011_20140620$},
pnm = {131 - Electrochemical Storage (POF3-131)},
pid = {G:(DE-HGF)POF3-131},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000439496500014},
doi = {10.1016/j.est.2018.04.029},
url = {https://juser.fz-juelich.de/record/866894},
}