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@ARTICLE{Bischof:866962,
author = {Bischof, Oliver and Weber, Patrick and Bundke, Ulrich and
Petzold, Andreas and Kiendler-Scharr, Astrid},
title = {{C}haracterization of the {M}iniaturized {I}nverted {F}lame
{B}urner as a {C}ombustion {S}ource to {G}enerate a
{N}anoparticle {C}alibration {A}erosol},
journal = {Emission control science and technology},
volume = {6},
number = {1},
issn = {2199-3629},
address = {Berlin [u.a.]},
publisher = {Springer},
reportid = {FZJ-2019-06009},
pages = {37 - 46},
year = {2019},
abstract = {Soot generators are able to produce carbonaceous
nanoparticles purposefully and can therefore play a vital
role in the calibration of particle instruments with an
actual combustion aerosol. Condensation particle counters
(CPCs) have become the instrument of choice for legislative
measurements of the particle number (PN) concentration. The
Euro 5B standard introduced by the European Union in 2011
was the first regulation that introduced a PN limit for the
exhaust emission from light duty diesel vehicles. Since
then, several other PN regulations for soot-emitting
vehicles and combustion engines have been introduced or are
currently in draft stages, all with similar requirements for
the periodic calibration of the particle counter’s
measurement accuracy. It is for this reason that combustion
particles produced under laboratory conditions have become
an attractive choice of calibration aerosol. Nonetheless, it
is often difficult to generate a large amount of particles
in the small nanometer range from a laboratory combustion
source. In this study, we evaluated the performance of a
recently introduced soot generator and its suitability for
calibrating the counting efficiency and lower cut-off size
of CPCs in the nanometer size range. We first characterized
the soot generator’s warm up time to determine when it
reaches a stable output when using propane as its fuel. We
then investigated the influence of a dozen propane-to-air
flow settings on the resulting particle size distribution of
the combustion aerosol. Finally, we determined the resulting
nanoparticle concentrations for 13 size classes below 20 nm
in order to achieve a high size resolution at or near the
lower detection limit of common CPCs. We performed our
measurements under low-pressure conditions as our group
operates CPCs onboard commercial passenger aircraft that are
used as an atmospheric measurement platform. Another
consideration is that CPCs are also operated elsewhere at
much less than standard sea-level pressure. Examples include
high-altitude research stations as well as engine test rigs
used for vehicle exhaust emission testing or certification
operated at elevated locations, e.g., in the USA, Mexico,
and China. From these experiments, we concluded that when
operating this novel soot generator with 7.5 SLPM airflow
and 62.5 SCPM propane flow, it is possible to generate a
realistic combustion aerosol for tests and calibrations that
is still adequate even in the small nanometer size range.
The concentrations measured under these operating conditions
were just sufficient for detection with an aerosol
electrometer, which is the concentration reference typically
used in CPC calibrations.},
cin = {IEK-8},
ddc = {333.7},
cid = {I:(DE-Juel1)IEK-8-20101013},
pnm = {243 - Tropospheric trace substances and their
transformation processes (POF3-243)},
pid = {G:(DE-HGF)POF3-243},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000703946700004},
doi = {10.1007/s40825-019-00147-w},
url = {https://juser.fz-juelich.de/record/866962},
}