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@ARTICLE{Jin:867698,
author = {Jin, W. T. and Meven, Martin and Deng, H. and Su, Y. and
Wu, W. and Julian, S. R. and Kim, Young-June},
title = {{S}pin reorientation in {F}e{C}r{A}s revealed by
single-crystal neutron diffraction},
journal = {Physical review / B},
volume = {100},
number = {17},
issn = {2469-9950},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {FZJ-2019-06313},
pages = {174421},
year = {2019},
abstract = {The magnetic structure of the “nonmetallic metal”
FeCrAs, a compound with the characters of both metals and
insulators, was examined as a function of temperature using
single-crystal neutron diffraction. The magnetic propagation
vector was found to be k=(1/3,1/3,0), and the magnetic
reflections disappeared above TN=116(1)K. In the ground
state, the Cr sublattice shows an in-plane spiral
antiferromagnetic order. The moment sizes of the Cr ions
were found to be small due to strong magnetic frustration in
the distorted kagome lattice or the itinerant nature of the
Cr magnetism and vary between 0.8 and 1.4μB on different
sites as expected for a spin-density-wave- (SDW-) type
order. The upper limit of the moment on the Fe sublattice is
estimated to be less than 0.1μB. With increasing
temperature up to 95 K, the Cr moments cant out of the ab
plane gradually with the in-plane components being
suppressed and the out-of-plane components increasing in
contrast. This spin reorientation of Cr moments can explain
the dip in the c-direction magnetic susceptibility and the
kink in the magnetic order parameter at TO∼100K, a second
magnetic transition which was ignored before. We have also
discussed the similarity between FeCrAs and the model
itinerant magnet Cr, which exhibits spin-flip transitions
and SDW-type antiferromagnetism.},
cin = {JCNS-FRM-II},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218},
pnm = {6212 - Quantum Condensed Matter: Magnetism,
Superconductivity (POF3-621) / 144 - Controlling Collective
States (POF3-144) / 6G4 - Jülich Centre for Neutron
Research (JCNS) (POF3-623) / 6G15 - FRM II / MLZ
(POF3-6G15)},
pid = {G:(DE-HGF)POF3-6212 / G:(DE-HGF)POF3-144 /
G:(DE-HGF)POF3-6G4 / G:(DE-HGF)POF3-6G15},
experiment = {EXP:(DE-MLZ)HEIDI-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000496923700003},
doi = {10.1103/PhysRevB.100.174421},
url = {https://juser.fz-juelich.de/record/867698},
}