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@ARTICLE{Jung:868386,
      author       = {Jung, Florian A. and Panteli, Panayiota A. and Ko,
                      Chia-Hsin and Kang, Jia-Jhen and Barnsley, Lester C. and
                      Tsitsilianis, Constantinos and Patrickios, Costas S. and
                      Papadakis, Christine M.},
      title        = {{S}tructural {P}roperties of {M}icelles {F}ormed by
                      {T}elechelic {P}entablock {Q}uaterpolymers with
                      p{H}-{R}esponsive {M}idblocks and {T}hermoresponsive {E}nd
                      {B}locks in {A}queous {S}olution},
      journal      = {Macromolecules},
      volume       = {52},
      number       = {24},
      issn         = {1520-5835},
      address      = {Washington, DC},
      publisher    = {Soc.},
      reportid     = {FZJ-2020-00002},
      pages        = {9746 - 9758},
      year         = {2019},
      abstract     = {We investigated the structural properties of dynamic
                      micelles arising from the self-assembly of the
                      multiresponsive pentablock quaterpolymer
                      P(nBuMA8-co-TEGMA8)-b-PDMAEMA50-b-PEG46-b-PDMAEMA50-b-P(nBuMA8-co-TEGMA8)
                      (nBuMA, TEGMA, DMAEMA, and EG are n-butyl methacrylate,
                      tri(ethylene glycol) methyl ether methacrylate,
                      2-(dimethylamino)ethyl methacrylate, and ethylene glycol,
                      respectively) in aqueous solution using a combination of
                      scattering methods. In this multisegmented polymer, a
                      pH-responsive BAB triblock copolymer from the weak cationic
                      polyelectrolyte PDMAEMA and the hydrophilic PEG is
                      end-capped by two blocks comprising random sequences of
                      thermoresponsive TEGMA units and hydrophobic nBuMA units.
                      Dynamic light scattering revealed the existence of single
                      micelles and small clusters in dilute aqueous solution. The
                      hydrodynamic radius of the micelles depends strongly on pH
                      and temperature. The inner structure of the micelles was
                      investigated by small-angle X-ray scattering, small-angle
                      neutron scattering, and static light scattering, and
                      micelles with a hydrophobic core containing a rather high
                      fraction of water and a strongly swollen corona were found.
                      The ratio of loops and dangling ends depends on temperature
                      and pH.},
      cin          = {JCNS-FRM-II / MLZ},
      ddc          = {540},
      cid          = {I:(DE-Juel1)JCNS-FRM-II-20110218 / I:(DE-588b)4597118-3},
      pnm          = {6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)
                      / 6G15 - FRM II / MLZ (POF3-6G15)},
      pid          = {G:(DE-HGF)POF3-6G4 / G:(DE-HGF)POF3-6G15},
      experiment   = {EXP:(DE-MLZ)KWS1-20140101},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000505629900035},
      doi          = {10.1021/acs.macromol.9b01775},
      url          = {https://juser.fz-juelich.de/record/868386},
}