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@ARTICLE{Klingberg:872611,
author = {Klingberg, Patrik and Wilkner, Kai and Schlüter, Markus
and Grünauer, Judith and Shishatskiy, Sergey},
title = {{S}eparation of {C}arbon {D}ioxide from {R}eal {P}ower
{P}lant {F}lue {G}ases by {G}as {P}ermeation {U}sing a
{S}upported {I}onic {L}iquid {M}embrane: {A}n
{I}nvestigation of {M}embrane {S}tability},
journal = {Membranes},
volume = {9},
number = {3},
issn = {2077-0375},
address = {Basel},
publisher = {MDPI},
reportid = {FZJ-2020-00104},
pages = {35 -},
year = {2019},
abstract = {The separation of carbon dioxide from coal-fired power
plant flue gases using a CO2/N2-selective supported ionic
liquid membrane (SILM) was investigated and the performance
and stability of the membrane during operation are reported.
The membrane is composed of a polyacrylonitrile (PAN)
ultrafiltration membrane as a support and a selective layer
of an ionic liquid (IL), 1-ethyl-3-methylimidazolium
bis(trifluoromethylsulfonyl)imide (EMIM Tf2N). The
feasibility of large-scale SILM production was demonstrated
by the formation of a square-meter-scale membrane and
preparation of a membrane module. A flat-sheet envelope-type
SILM module containing 0.67 m2 of the membrane was
assembled. Prior to real flue gas operation, the separation
behaviour of the membrane was investigated with single
gases. The stability of the SILM during the test stand and
pilot plant operation using real power plant flue gases is
reported. The volume fraction of carbon dioxide in the flue
gas was raised from approx. 14 vol. $\%$ (feed) to 40 vol.
$\%$ (permeate). However, issues concerning the membrane
stability were found when SO3 aerosols in large quantities
were present in the flue gas},
cin = {IEK-1},
ddc = {570},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {113 - Methods and Concepts for Material Development
(POF3-113)},
pid = {G:(DE-HGF)POF3-113},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:30836621},
UT = {WOS:000464144000001},
doi = {10.3390/membranes9030035},
url = {https://juser.fz-juelich.de/record/872611},
}