000872615 001__ 872615
000872615 005__ 20230426083218.0
000872615 0247_ $$2doi$$a10.1103/PhysRevB.101.024103
000872615 0247_ $$2ISSN$$a0163-1829
000872615 0247_ $$2ISSN$$a0556-2805
000872615 0247_ $$2ISSN$$a1050-2947
000872615 0247_ $$2ISSN$$a1094-1622
000872615 0247_ $$2ISSN$$a1095-3795
000872615 0247_ $$2ISSN$$a1098-0121
000872615 0247_ $$2ISSN$$a1538-4489
000872615 0247_ $$2ISSN$$a1550-235X
000872615 0247_ $$2ISSN$$a2469-9950
000872615 0247_ $$2ISSN$$a2469-9969
000872615 0247_ $$2Handle$$a2128/23822
000872615 0247_ $$2altmetric$$aaltmetric:73910728
000872615 0247_ $$2WOS$$aWOS:000506583800003
000872615 037__ $$aFZJ-2020-00108
000872615 082__ $$a530
000872615 1001_ $$0P:(DE-Juel1)130741$$aJones, Robert O.$$b0$$eCorresponding author
000872615 245__ $$aPhase change memory materials: Rationalizing the dominance of Ge/Sb/Te alloys
000872615 260__ $$aWoodbury, NY$$bInst.$$c2020
000872615 3367_ $$2DRIVER$$aarticle
000872615 3367_ $$2DataCite$$aOutput Types/Journal article
000872615 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1579694797_19654
000872615 3367_ $$2BibTeX$$aARTICLE
000872615 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000872615 3367_ $$00$$2EndNote$$aJournal Article
000872615 520__ $$aRewritable optical storage is dominated by alloys of a small number of elements, overwhelmingly Ge, Sb, and Te. For over 30 years, Ge/Sb/Te alloys in the composition range (GeTe)1−x(Sb2Te3)x(0≤x≤1) have been the materials of choice in commercial devices: all have metastable rock-salt structures that change little over decades at archival temperatures, and all contain vacancies (cavities). The special status of Ge/Sb/Te alloys arises from the close similarity of their valence orbitals as measured by the orbital radial moments, so that bonds are stronger than in other combinations of elements of groups 14–16 with appropriate valences. The orbital similarity arises from the irregular changes in atomic orbitals and properties as the atomic number increases (“secondary periodicity”). Jones showed [P. R. Soc. London, Ser. A 147, 396 (1934)] that the simple cubic structure of (metallic) Bi (valence configuration 6s26p3) is unstable to a distortion to a (semimetallic) rhombohedral structure. This picture can be adapted to Ge/Sb/Te alloys to explain the metastable structure of the above family of compounds where vacancies almost always occur next to Te atoms, which form one sublattice of the rock-salt structure. The disorder in the Ge/Sb/vacancy sublattice is not random.
000872615 536__ $$0G:(DE-HGF)POF3-142$$a142 - Controlling Spin-Based Phenomena (POF3-142)$$cPOF3-142$$fPOF III$$x0
000872615 536__ $$0G:(DE-HGF)POF3-143$$a143 - Controlling Configuration-Based Phenomena (POF3-143)$$cPOF3-143$$fPOF III$$x1
000872615 536__ $$0G:(DE-Juel1)jiff05_20170501$$aDensity functional calculations with molecular dynamics -- amorphous and crystalline materials (jiff05_20170501)$$cjiff05_20170501$$fDensity functional calculations with molecular dynamics -- amorphous and crystalline materials$$x2
000872615 542__ $$2Crossref$$i2020-01-09$$uhttps://link.aps.org/licenses/aps-default-license
000872615 588__ $$aDataset connected to CrossRef
000872615 77318 $$2Crossref$$3journal-article$$a10.1103/physrevb.101.024103$$bAmerican Physical Society (APS)$$d2020-01-09$$n2$$p024103$$tPhysical Review B$$v101$$x2469-9950$$y2020
000872615 773__ $$0PERI:(DE-600)2844160-6$$a10.1103/PhysRevB.101.024103$$gVol. 101, no. 2, p. 024103$$n2$$p024103$$tPhysical review / B$$v101$$x2469-9950$$y2020
000872615 8564_ $$uhttps://juser.fz-juelich.de/record/872615/files/GSTx.pdf$$yOpenAccess
000872615 8564_ $$uhttps://juser.fz-juelich.de/record/872615/files/PhysRevB.101.024103.pdf$$yOpenAccess
000872615 8564_ $$uhttps://juser.fz-juelich.de/record/872615/files/GSTx.pdf?subformat=pdfa$$xpdfa$$yOpenAccess
000872615 8564_ $$uhttps://juser.fz-juelich.de/record/872615/files/PhysRevB.101.024103.pdf?subformat=pdfa$$xpdfa$$yOpenAccess
000872615 909CO $$ooai:juser.fz-juelich.de:872615$$pdnbdelivery$$pdriver$$pVDB$$popen_access$$popenaire
000872615 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130741$$aForschungszentrum Jülich$$b0$$kFZJ
000872615 9131_ $$0G:(DE-HGF)POF3-142$$1G:(DE-HGF)POF3-140$$2G:(DE-HGF)POF3-100$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$aDE-HGF$$bEnergie$$lFuture Information Technology - Fundamentals, Novel Concepts and Energy Efficiency (FIT)$$vControlling Spin-Based Phenomena$$x0
000872615 9131_ $$0G:(DE-HGF)POF3-143$$1G:(DE-HGF)POF3-140$$2G:(DE-HGF)POF3-100$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$aDE-HGF$$bEnergie$$lFuture Information Technology - Fundamentals, Novel Concepts and Energy Efficiency (FIT)$$vControlling Configuration-Based Phenomena$$x1
000872615 9141_ $$y2020
000872615 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS
000872615 915__ $$0StatID:(DE-HGF)0600$$2StatID$$aDBCoverage$$bEbsco Academic Search
000872615 915__ $$0LIC:(DE-HGF)APS-112012$$2HGFVOC$$aAmerican Physical Society Transfer of Copyright Agreement
000872615 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bPHYS REV B : 2017
000872615 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection
000872615 915__ $$0StatID:(DE-HGF)0110$$2StatID$$aWoS$$bScience Citation Index
000872615 915__ $$0StatID:(DE-HGF)0111$$2StatID$$aWoS$$bScience Citation Index Expanded
000872615 915__ $$0StatID:(DE-HGF)9900$$2StatID$$aIF < 5
000872615 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess
000872615 915__ $$0StatID:(DE-HGF)0030$$2StatID$$aPeer Review$$bASC
000872615 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences
000872615 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline
000872615 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bClarivate Analytics Master Journal List
000872615 9201_ $$0I:(DE-Juel1)IAS-1-20090406$$kIAS-1$$lQuanten-Theorie der Materialien$$x0
000872615 9201_ $$0I:(DE-Juel1)PGI-1-20110106$$kPGI-1$$lQuanten-Theorie der Materialien$$x1
000872615 9201_ $$0I:(DE-82)080012_20140620$$kJARA-HPC$$lJARA - HPC$$x2
000872615 980__ $$ajournal
000872615 980__ $$aVDB
000872615 980__ $$aI:(DE-Juel1)IAS-1-20090406
000872615 980__ $$aI:(DE-Juel1)PGI-1-20110106
000872615 980__ $$aI:(DE-82)080012_20140620
000872615 980__ $$aUNRESTRICTED
000872615 9801_ $$aFullTexts
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.21.1450
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1117/12.936065
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.97617
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1143/JJAP.43.4704
000872615 999C5 $$1N. K. Abrikosov$$2Crossref$$oN. K. Abrikosov 1965$$y1965
000872615 999C5 $$1N. K. Abrikosov$$2Crossref$$oN. K. Abrikosov 1965$$y1965
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1007/BF02758595
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.83.144205
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1039/C5TC02314A
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.4950817
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1007/s10825-017-1097-1
000872615 999C5 $$1N. Yamada$$2Crossref$$9-- missing cx lookup --$$a10.7567/JJAPS.26S4.61$$p61 -$$tJpn. J. Appl. Phys.$$v26$$y1987
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.348620
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1002/pssb.201200618
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1557/S0883769400036368
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1021/ic051677w
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.1502915
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1107/S0108768104022906
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1088/1361-6528/28/6/065706
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.79.134118
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1039/C7NR01684K
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1126/science.aao3212
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1126/science.aaq0476
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1038/s41563-018-0110-9
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1080/01611598308244064
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1038/nmat2330
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.86.144113
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.90.184109
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.94.134105
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1002/adfm.201500849
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1021/acs.jpcb.8b06476
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1088/1361-648X/aab22e
000872615 999C5 $$1L. Pauling$$2Crossref$$oL. Pauling The Nature of the Chemical Bond 1960$$tThe Nature of the Chemical Bond$$y1960
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.1749394
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.2.2147
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.33.1095
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.10.3316
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.24.2903
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.20.4082
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1088/0022-3719/13/26/009
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1002/adma.201806280
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRev.37.481
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1021/ja01355a027
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/RevModPhys.87.897
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.77.3865
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.40.2980
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.18.2701
000872615 999C5 $$1E. V. Biron$$2Crossref$$oE. V. Biron 1915$$y1915
000872615 999C5 $$1S. A. Shchukarev$$2Crossref$$oS. A. Shchukarev 1954$$y1954
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1039/PS9610000273
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1021/cr00085a006
000872615 999C5 $$1V. M. Goldschmidt$$2Crossref$$oV. M. Goldschmidt 1925$$y1925
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.465363
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevA.19.1813
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1016/j.tsf.2006.11.159
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1002/adma.200306077
000872615 999C5 $$1J. Donohue$$2Crossref$$oJ. Donohue The Structures of the Elements 1974$$tThe Structures of the Elements$$y1974
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.458306
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.467213
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.4983219
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1002/andp.19303960202
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1007/BF01339455
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1051/jphysrad:01930001011037700
000872615 999C5 $$1J. M. Ziman$$2Crossref$$oJ. M. Ziman Electrons and Phonons: The Theory of Transport Phenomena in Solids 1960$$tElectrons and Phonons: The Theory of Transport Phenomena in Solids$$y1960
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1098/rspa.1934.0224
000872615 999C5 $$1N. F. Mott$$2Crossref$$oN. F. Mott The Theory of the Properties of Metals and Alloys 1936$$tThe Theory of the Properties of Metals and Alloys$$y1936
000872615 999C5 $$1R. E. Peierls$$2Crossref$$oR. E. Peierls Quantum Theory of Solids 1955$$tQuantum Theory of Solids$$y1955
000872615 999C5 $$1H. Jones$$2Crossref$$oH. Jones The Theory of Brillouin Zones and Electronic States in Crystals 1975$$tThe Theory of Brillouin Zones and Electronic States in Crystals$$y1975
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1088/0022-3719/2/4/316
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1016/0038-1098(72)90551-0
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1016/0038-1098(92)90102-F
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1147/rd.83.0215
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.60.15484
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1051/jphyscol:1968410
000872615 999C5 $$1H. M. Polatoglou$$2Crossref$$oH. M. Polatoglou Physics of Narrow Gap Semiconductors 1982$$tPhysics of Narrow Gap Semiconductors$$y1982
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1016/j.crhy.2015.12.009
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.85.1950
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1088/0953-8984/20/46/465103
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1143/JJAP.44.7340
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1515/zpch-1897-2233
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1515/zpch-1933-16335
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1021/jp4031199
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1021/op030026l
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.3655358
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1021/j150668a002
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1039/a809346f
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1021/acs.cgd.9b00217
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1021/jp111835z
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1126/science.aaw1773
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.76.235201
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.100.205502
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.108.195506
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.4949011
000872615 999C5 $$1L. Pauling$$2Crossref$$oL. Pauling General Chemistry 1970$$tGeneral Chemistry$$y1970
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1038/nmat2226
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1038/srep13698
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1002/adma.201803777
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.81.081204
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1038/srep25981
000872615 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/RevModPhys.34.326