Hauptseite > Publikationsdatenbank > Partial Up-Up-Down Order with the Continuously Distributed Order Parameter in the Triangular Antiferromagnet TmMgGaO 4 > print

001     872664
005     20250129094203.0
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100 1 _ |a Li, Yuesheng
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245 _ _ |a Partial Up-Up-Down Order with the Continuously Distributed Order Parameter in the Triangular Antiferromagnet TmMgGaO 4
260 _ _ |a College Park, Md.
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520 _ _ |a We show that frustrated quasidoublets without time-reversal symmetry can host highly unconventional magnetic structures with continuously distributed order parameters even in a single-phase crystal. Our study comprises a comprehensive thermodynamic and neutron diffraction investigation on the single crystal of TmMgGaO4, which entails non-Kramers Tm3+ ions arranged on a geometrically perfect triangular lattice. The crystal electric field randomness caused by the site-mixing disorder of the nonmagnetic Mg2+ and Ga3+ ions merges two lowest-lying crystal electric field singlets of Tm3+ into a ground-state quasidoublet. Well below Tc∼0.7  K, a small fraction of the antiferromagnetically coupled Tm3+ Ising quasidoublets with small inner gaps condense into two-dimensional up-up-down magnetic structures with continuously distributed order parameters, and give rise to the columnar magnetic neutron reflections below μ0Hc∼2.6  T, with highly anisotropic correlation lengths, ξab≥250a in the triangular plane and ξc
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700 1 _ |a Bachus, Sebastian
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700 1 _ |a Deng, Hao
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773 _ _ |a 10.1103/PhysRevX.10.011007
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