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000872806 1001_ $$0P:(DE-Juel1)129898$$aPasel, Joachim$$b0$$eCorresponding author
000872806 245__ $$aCombined near-ambient pressure photoelectron spectroscopy and temporal analysis of products study of CH4 oxidation on Pd/γ-Al2O3 catalysts
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000872806 520__ $$aVehicles that run on natural gas must be equipped with an exhaust gas after-treatment system to burn their unavoidable CH4 slip, which must not be released into the environment as CH4 is a potent greenhouse gas. Pd is known as a highly active catalyst material for CH4 oxidation. For this study, Pd was deposited on a γ-Al2O3 support and the as-received samples were pre-reduced and pre-oxidized, respectively. Near-Ambient Pressure Photoelectron Spectroscopy and the Temporal Analysis of Products methodology were combined to understand that both electronic states, namely PdO and Pd°, are active for the CH4 oxidation reaction, whereby the superior activity of the pre-reduced Pd/γ-Al2O3 catalyst was ascribed to the spill-over of OH-groups from the support to Pd. It was found that the reaction products, CO, CO2 and H2, were strongly and, to a large extent, adsorbed on the catalyst surface and were involved in reversible chemical interactions on the catalyst surface during the CH4 oxidation reaction on the Pd/γ-Al2O3 catalyst.
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000872806 7001_ $$0P:(DE-Juel1)129920$$aSchmitt, Dirk$$b1
000872806 7001_ $$0P:(DE-Juel1)166271$$aHartmann, Heinrich$$b2
000872806 7001_ $$0P:(DE-Juel1)133839$$aBesmehn, Astrid$$b3
000872806 7001_ $$0P:(DE-Juel1)129189$$aDornseiffer, Jürgen$$b4
000872806 7001_ $$0P:(DE-Juel1)162457$$aWerner, Jonas$$b5
000872806 7001_ $$0P:(DE-Juel1)130824$$aMayer, Joachim$$b6
000872806 7001_ $$0P:(DE-Juel1)129902$$aPeters, Ralf$$b7
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000872806 773__ $$0PERI:(DE-600)2012626-8$$a10.1016/j.cattod.2019.12.026$$gp. S0920586119306753$$p444-453$$tCatalysis today$$v360$$x0920-5861$$y2021
000872806 8564_ $$uhttps://juser.fz-juelich.de/record/872806/files/Pasel_Joachim_2019_CATTOD.pdf$$yPublished on 2019-12-26. Available in OpenAccess from 2020-12-26.
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