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@ARTICLE{Pasel:872806,
      author       = {Pasel, Joachim and Schmitt, Dirk and Hartmann, Heinrich and
                      Besmehn, Astrid and Dornseiffer, Jürgen and Werner, Jonas
                      and Mayer, Joachim and Peters, Ralf},
      title        = {{C}ombined near-ambient pressure photoelectron spectroscopy
                      and temporal analysis of products study of {CH}4 oxidation
                      on {P}d/γ-{A}l2{O}3 catalysts},
      journal      = {Catalysis today},
      volume       = {360},
      issn         = {0920-5861},
      address      = {Amsterdam},
      publisher    = {Elsevier},
      reportid     = {FZJ-2020-00278},
      pages        = {444-453},
      year         = {2021},
      abstract     = {Vehicles that run on natural gas must be equipped with an
                      exhaust gas after-treatment system to burn their unavoidable
                      CH4 slip, which must not be released into the environment as
                      CH4 is a potent greenhouse gas. Pd is known as a highly
                      active catalyst material for CH4 oxidation. For this study,
                      Pd was deposited on a γ-Al2O3 support and the as-received
                      samples were pre-reduced and pre-oxidized, respectively.
                      Near-Ambient Pressure Photoelectron Spectroscopy and the
                      Temporal Analysis of Products methodology were combined to
                      understand that both electronic states, namely PdO and Pd°,
                      are active for the CH4 oxidation reaction, whereby the
                      superior activity of the pre-reduced Pd/γ-Al2O3 catalyst
                      was ascribed to the spill-over of OH-groups from the support
                      to Pd. It was found that the reaction products, CO, CO2 and
                      H2, were strongly and, to a large extent, adsorbed on the
                      catalyst surface and were involved in reversible chemical
                      interactions on the catalyst surface during the CH4
                      oxidation reaction on the Pd/γ-Al2O3 catalyst.},
      cin          = {IEK-14 / ZEA-3 / ER-C-2},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-14-20191129 / I:(DE-Juel1)ZEA-3-20090406 /
                      I:(DE-Juel1)ER-C-2-20170209},
      pnm          = {135 - Fuel Cells (POF3-135) / 131 - Electrochemical Storage
                      (POF3-131) / 1232 - Power-based Fuels and Chemicals
                      (POF4-123)},
      pid          = {G:(DE-HGF)POF3-135 / G:(DE-HGF)POF3-131 /
                      G:(DE-HGF)POF4-1232},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000594832500006},
      doi          = {10.1016/j.cattod.2019.12.026},
      url          = {https://juser.fz-juelich.de/record/872806},
}