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| Hauptseite > Publikationsdatenbank > Combined near-ambient pressure photoelectron spectroscopy and temporal analysis of products study of CH4 oxidation on Pd/γ-Al2O3 catalysts > print |
| Hauptseite > Publikationsdatenbank > Combined near-ambient pressure photoelectron spectroscopy and temporal analysis of products study of CH4 oxidation on Pd/γ-Al2O3 catalysts > print |
| 001 | 872806 | ||
| 005 | 20240709082046.0 | ||
| 024 | 7 | _ | |a 10.1016/j.cattod.2019.12.026 |2 doi |
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| 037 | _ | _ | |a FZJ-2020-00278 |
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| 100 | 1 | _ | |a Pasel, Joachim |0 P:(DE-Juel1)129898 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Combined near-ambient pressure photoelectron spectroscopy and temporal analysis of products study of CH4 oxidation on Pd/γ-Al2O3 catalysts |
| 260 | _ | _ | |a Amsterdam |c 2021 |b Elsevier |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Vehicles that run on natural gas must be equipped with an exhaust gas after-treatment system to burn their unavoidable CH4 slip, which must not be released into the environment as CH4 is a potent greenhouse gas. Pd is known as a highly active catalyst material for CH4 oxidation. For this study, Pd was deposited on a γ-Al2O3 support and the as-received samples were pre-reduced and pre-oxidized, respectively. Near-Ambient Pressure Photoelectron Spectroscopy and the Temporal Analysis of Products methodology were combined to understand that both electronic states, namely PdO and Pd°, are active for the CH4 oxidation reaction, whereby the superior activity of the pre-reduced Pd/γ-Al2O3 catalyst was ascribed to the spill-over of OH-groups from the support to Pd. It was found that the reaction products, CO, CO2 and H2, were strongly and, to a large extent, adsorbed on the catalyst surface and were involved in reversible chemical interactions on the catalyst surface during the CH4 oxidation reaction on the Pd/γ-Al2O3 catalyst. |
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| 536 | _ | _ | |a 1232 - Power-based Fuels and Chemicals (POF4-123) |0 G:(DE-HGF)POF4-1232 |c POF4-123 |f POF IV |x 2 |
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| 773 | _ | _ | |a 10.1016/j.cattod.2019.12.026 |g p. S0920586119306753 |0 PERI:(DE-600)2012626-8 |p 444-453 |t Catalysis today |v 360 |y 2021 |x 0920-5861 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/872806/files/Pasel_Joachim_2019_CATTOD.pdf |y Published on 2019-12-26. Available in OpenAccess from 2020-12-26. |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/872806/files/Pasel_Joachim_2019_CATTOD.pdf?subformat=pdfa |x pdfa |y Published on 2019-12-26. Available in OpenAccess from 2020-12-26. |
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