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@ARTICLE{Kutovyi:873640,
author = {Kutovyi, Yurii and Hlukhova, Hanna and Boichuk, Nazarii and
Menger, Marcus and Offenhäusser, Andreas and Vitusevich,
Svetlana},
title = {{A}myloid-beta peptide detection via aptamer-functionalized
nanowire sensors exploiting single-trap phenomena},
journal = {Biosensors and bioelectronics},
volume = {154},
issn = {0956-5663},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2020-00883},
pages = {112053 -1-8},
year = {2020},
abstract = {New highly sensitive direct methods for the early detection
of peptides involved in Alzheimer's disease (AD) are
required in order to prolong effective and healthy memory
and thinking capabilities and also to stop the factors
resulting in AD. In this contribution, we report the
successful demonstration of a label-free approach for the
detection of amyloid-beta (Aβ) peptides by highly selective
aptamers immobilized onto the SiO2 surface of the fabricated
sensors. A modified single-stranded deoxyribonucleic acid
(ssDNA) aptamer was specially designed and synthesized to
detect the target amyloid beta-40 sequence (Aβ-40).
Electrolyte–insulator–semiconductor (EIS) structures as
well as silicon (Si) nanowire (NW) field-effect transistors
(FETs) covered with a thin SiO2 dielectric layer have been
successfully functionalized with Aβ-40-specific aptamers
and used to detect ultra-low concentrations of the target
peptide. The binding of amyloid-beta peptides of different
concentrations to the surface of the sensors varied in the
range from 0.1 pg/ml to 10 μg/ml resulting in a change of
the surface potential was registered by the fabricated
devices. Moreover, we show that the single-trap phenomena
observed in the novel Si two-layer (TL) NW FET structures
with advanced characteristic parameters can be effectively
used to increase the sensitivity of nanoscale sensors. The
obtained experimental data demonstrate a highly sensitive
and reliable detection of ultra-low concentrations of the
Aβ-40 peptides. This opens up prospects for the development
of real-time electrical biosensors for studying and
understanding different stages of AD by utilizing Si TL NW
FET structures fabricated on the basis of cost-efficient
CMOS-compatible technology.},
cin = {IBI-3},
ddc = {610},
cid = {I:(DE-Juel1)IBI-3-20200312},
pnm = {5241 - Molecular Information Processing in Cellular Systems
(POF4-524)},
pid = {G:(DE-HGF)POF4-5241},
typ = {PUB:(DE-HGF)16},
pubmed = {32056959},
UT = {WOS:000519667000006},
doi = {10.1016/j.bios.2020.112053},
url = {https://juser.fz-juelich.de/record/873640},
}