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@ARTICLE{Xu:873869,
author = {Xu, Liangfei and Fang, Chuan and Li, Jianqiu and Ouyang,
Minggao and Lehnert, Werner},
title = {{N}onlinear dynamic mechanism modeling of a polymer
electrolyte membrane fuel cell with dead-ended anode
considering mass transport and actuator properties},
journal = {Applied energy},
volume = {230},
issn = {0306-2619},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2020-01061},
pages = {106 - 121},
year = {2018},
abstract = {A dead-ended anode (DEA) has advantages such as simple
structure, high reliability, and low price, and is widely
utilized in polymer electrolyte membrane fuel cell (PEMFC)
systems. Empirical parameters are commonly adopted in
control-oriented models for such systems, and detailed
information about mass transport processes is usually not
available. Such models are neither helpful for understanding
the internal processes within fuel cells, nor for designing
control algorithms to improve system performance. A
control-oriented model considering the mass transport
processes and actuator properties is still lacking. This
paper proposes a nonlinear dynamic mechanism model for the
DEA system that can describe the dynamic voltage drop during
water flooding with a large current density. The properties
of the major components are explained in details, and the
procedure of how the purging valves affects the mass
transport and cell voltage is revealed quantitatively. The
relationship between the minimum cell voltage and purging
operations is summarized. The results show that (1) the
proposed model can capture the stable and dynamic properties
of a fuel cell with a DEA, (2) the cell voltage loss during
closing of the purging valve is mainly caused by a decrease
in oxygen and hydrogen partial pressures on the catalyst
layers and an increase in the liquid water saturation ratio
in the gas diffusion layers (GDLs); (3) the most important
internal states that affect the stack voltage during purging
is the liquid water saturation ratio in the GDLs.},
cin = {IEK-14 / IEK-3},
ddc = {620},
cid = {I:(DE-Juel1)IEK-14-20191129 / I:(DE-Juel1)IEK-3-20101013},
pnm = {135 - Fuel Cells (POF3-135)},
pid = {G:(DE-HGF)POF3-135},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000448226600010},
doi = {10.1016/j.apenergy.2018.08.099},
url = {https://juser.fz-juelich.de/record/873869},
}