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@ARTICLE{Koslowski:874010,
author = {Koslowski, Hans Rudolf and Schmitz, Janina and Linsmeier,
Christian},
title = {{S}egregation and {P}referential {S}puttering of {C}r in
{WC}r{Y} {S}mart {A}lloy},
journal = {Nuclear materials and energy},
volume = {22},
issn = {2352-1791},
address = {Amsterdam [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2020-01170},
pages = {100736 -},
year = {2020},
abstract = {The temperature driven segregation of Cr to the surface of
the tungsten-based WCrY alloy is analysed with low energy
ion scattering of He+ ions with an energy of 1 keV in the
temperature range from room temperature to 1000 K. Due to
the high surface sensitivity, these measurements probe only
the composition of the outermost monolayer. The surface
concentration of Cr increases slightly when the temperature
of the sample is increased up to 700 K and exhibits a much
stronger increase when the sample temperature is further
raised. The segregation enthalpy for Cr is obtained from the
Langmuir-McLean relation and amounts to 0.7 eV. The
surface concentration of Y shows a similar behaviour to the
Cr concentration. The temperature thresholds between slow
and accelerated surface density increases for Cr and Y are
nearly the same. At a temperature of 1000 K the low energy
ion scattering detects almost no W on the surface. The
modified surface composition due to the segregated species,
i.e. the mixed Cr/Y layer, stays stable during cool-down of
the sample. Preferential sputtering is investigated using
ion bombardment of 250 eV D atoms, resulting in an
increase of the W surface density at room temperature. This
effect is counteracted at elevated temperatures where
segregation replenishes the lighter elements on the surface
and prevents the formation of an all-W surface layer. The
flux of segregating Cr atoms towards the surface is
evaluated from the equilibrium between sputter erosion and
segregation.},
cin = {IEK-4},
ddc = {624},
cid = {I:(DE-Juel1)IEK-4-20101013},
pnm = {113 - Methods and Concepts for Material Development
(POF3-113)},
pid = {G:(DE-HGF)POF3-113},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000525256600020},
doi = {10.1016/j.nme.2020.100736},
url = {https://juser.fz-juelich.de/record/874010},
}