Home > Publications database > Covalent triazine framework/carbon nanotube hybrids enabling selective reduction of CO 2 to CO at low overpotential > print

001     877538
005     20210130005113.0
024 7 _ |a 10.1039/D0GC00090F
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100 1 _ |a Laemont, Andreas
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245 _ _ |a Covalent triazine framework/carbon nanotube hybrids enabling selective reduction of CO 2 to CO at low overpotential
260 _ _ |a Cambridge
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520 _ _ |a Electrochemical reduction of CO2 provides a way to generate base chemicals from an abundant C1-source under mild conditions, whilst at the same time mitigating CO2 emissions. In this work, a novel class of tailorable, porous electrocatalysts for this process is proposed. Covalent triazine frameworks (CTFs) are grown in situ onto functionalized multiwalled carbon nanotubes. Hydroxyl groups decorating the surface of the multiwalled carbon nanotubes facilitate intimate contact between the carbon nanotubes and CTF, thus promoting efficient electron transfer. The novel hybrid materials generate CO with a faradaic efficiency up to 81% at an overpotential of 380 mV. The selectivity of the electrocatalysts could be linked to the amount of nitrogen present within the framework.
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700 1 _ |a Abednatanzi, Sara
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700 1 _ |a Derakshandeh, Parviz Gohari
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700 1 _ |a Verbruggen, Florian
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700 1 _ |a Fiset, Erika
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700 1 _ |a Qin, Qing
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700 1 _ |a Van Daele, Kevin
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700 1 _ |a Meledina, Maria
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700 1 _ |a Schmidt, Johannes
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700 1 _ |a Oschatz, Martin
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700 1 _ |a Van Der Voort, Pascal
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700 1 _ |a Rabaey, Korneel
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700 1 _ |a Antonietti, Markus
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700 1 _ |a Breugelmans, Tom
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700 1 _ |a Leus, Karen
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|e Corresponding author
773 _ _ |a 10.1039/D0GC00090F
|g Vol. 22, no. 10, p. 3095 - 3103
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|t Green chemistry
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|y 2020
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856 4 _ |u https://juser.fz-juelich.de/record/877538/files/d0gc00090f.pdf
856 4 _ |y Published on 2020-02-13. Available in OpenAccess from 2021-02-13.
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856 4 _ |y Published on 2020-02-13. Available in OpenAccess from 2021-02-13.
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