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@ARTICLE{Ktelhn:877617,
author = {Kätelhön, Arne and Meys, Raoul and Deutz, Sarah and Suh,
Sangwon and Bardow, André},
title = {{C}limate change mitigation potential of carbon capture and
utilization in the chemical industry},
journal = {Proceedings of the National Academy of Sciences of the
United States of America},
volume = {116},
number = {23},
issn = {1091-6490},
address = {Washington, DC},
publisher = {National Acad. of Sciences},
reportid = {FZJ-2020-02332},
pages = {11187 - 11194},
year = {2019},
abstract = {Chemical production is set to become the single largest
driver of global oil consumption by 2030. To reduce oil
consumption and resulting greenhouse gas (GHG) emissions,
carbon dioxide can be captured from stacks or air and
utilized as alternative carbon source for chemicals. Here,
we show that carbon capture and utilization (CCU) has the
technical potential to decouple chemical production from
fossil resources, reducing annual GHG emissions by up to 3.5
Gt CO2-eq in 2030. Exploiting this potential, however,
requires more than 18.1 PWh of low-carbon electricity,
corresponding to $55\%$ of the projected global electricity
production in 2030. Most large-scale CCU technologies are
found to be less efficient in reducing GHG emissions per
unit low-carbon electricity when benchmarked to power-to-X
efficiencies reported for other large-scale applications
including electro-mobility (e-mobility) and heat pumps. Once
and where these other demands are satisfied, CCU in the
chemical industry could efficiently contribute to climate
change mitigation.},
cin = {IEK-10},
ddc = {500},
cid = {I:(DE-Juel1)IEK-10-20170217},
pnm = {899 - ohne Topic (POF3-899)},
pid = {G:(DE-HGF)POF3-899},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:31085651},
UT = {WOS:000470136000023},
doi = {10.1073/pnas.1821029116},
url = {https://juser.fz-juelich.de/record/877617},
}