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@ARTICLE{Tsai:877719,
author = {Tsai, Chih-Long and Yu, Shicheng and Tempel, Hermann and
Kungl, Hans and Eichel, Rüdiger-A.},
title = {{A}ll-ceramic {L}i batteries based on garnet structured
{L}i 7 {L}a 3 {Z}r 2 {O} 12},
journal = {Materials technology},
volume = {35},
number = {9-10},
issn = {1753-5557},
address = {London},
publisher = {Taylor and Francis},
reportid = {FZJ-2020-02420},
pages = {656-674},
year = {2020},
abstract = {All-ceramic Li batteries (CLBs) are expected as next
generation energy storage devices because of their potential
to have higher energy density and safety than nowadays
Li-ion batteries. Garnet structured Li7La3Zr2O12 (LLZO)
plays an important role on CLB developments due to its fast
Li-ion conductivity, intrinsic stability toward Li and high
chemical and electrochemical stabilities. After a decade of
researches, many problems have been answered for LLZO-based
CLB developments but still numerous challenges left to be
solved. This review presents the latest efforts on the
development of LLZO based CLBs, which covers the advances in
LLZO crystal structure to increase its ionic conductivity
and progresses in the use of Li as the electrode, regarding
to its intrinsic chemical stability toward Li and interface
elaboration for allowing Li dendrite suppression. On the
positive electrode developments, chemical compatibility of
various active materials and strategies to circumvent the
incompatibility issue at high sintering temperatures are
inspected.},
cin = {IEK-9 / IEK-12},
ddc = {600},
cid = {I:(DE-Juel1)IEK-9-20110218 / I:(DE-Juel1)IEK-12-20141217},
pnm = {131 - Electrochemical Storage (POF3-131)},
pid = {G:(DE-HGF)POF3-131},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000538739800001},
doi = {10.1080/10667857.2020.1746539},
url = {https://juser.fz-juelich.de/record/877719},
}