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100 1 _ |a Chen, Lebing
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245 _ _ |a Magnetic anisotropy in ferromagnetic CrI 3
260 _ _ |a Woodbury, NY
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520 _ _ |a We use neutron scattering to show that ferromagnetic (FM) phase transition in the two-dimensional (2D)honeycomb lattice CrI3 is a weakly first order transition and controlled by spin-orbit coupling (SOC) inducedmagnetic anisotropy, instead of magnetic exchange coupling as in a conventional ferromagnet. With increasingtemperature, the magnitude of magnetic anisotropy, seen as a spin gap at the Brillouin zone center, decreasesin a power law fashion and vanishes at TC, while the in-plane and c-axis spin-wave stiffnesses associated withmagnetic exchange couplings remain robust at TC.We also compare parameter regimes where spin waves in CrI3can be described by a Heisenberg Hamiltonian with Dzyaloshinskii-Moriya interaction or a Heisenberg-KitaevHamiltonian. These results suggest that the SOC induced magnetic anisotropy plays a dominant role in stabilizingthe FM order in single layer 2D van der Waals ferromagnets.
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700 1 _ |a Chung, Jae-Ho
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700 1 _ |a Chen, Tong
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700 1 _ |a Duan, Chunruo
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700 1 _ |a Schneidewind, Astrid
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700 1 _ |a Kolesnikov, Alexander I.
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700 1 _ |a Chi, Songxue
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700 1 _ |a Mole, R. A.
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700 1 _ |a Yu, D. H.
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700 1 _ |a Gao, Bin
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700 1 _ |a Dai, Pengcheng
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773 _ _ |a 10.1103/PhysRevB.101.134418
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