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@ARTICLE{Moradabadi:878028,
author = {Moradabadi, Ashkan and Kaghazchi, Payam},
title = {{E}ffect of lattice and dopant–induced strain on the
conductivity of solid electrolytes: application of the
elastic dipole method},
journal = {Materialia},
volume = {9},
issn = {2589-1529},
address = {Amsterdam},
publisher = {Elsevier},
reportid = {FZJ-2020-02584},
pages = {100607},
year = {2020},
abstract = {Here, we studied the possibility of applying the elastic
dipole method (EDM) to predict the response of defect
formation and migration energy to an external strain field
(ϵij) in Al-doped cubic Li6.25Al0.25La3Zr2O12 (Al-LLZO) and
Li10GeP2S12 (LGPS). It is shown that EDM can quantitatively
provide accurate values for Li-defect formation energy as a
function of ϵij. EDM can also predict, qualitatively, how
the migration barrier varies with ϵij. In both Al-LLZO and
LGPS systems, the formation energy of Li vacancy decreases
(increases) by applying a tensile (compressive) strain,
which is because the lattice parameters tend to expand by
formation of a Li vacancy. An opposite behavior is found for
the formation energy of interstitial Li. Furthermore, we
found that a compressive strain decreases the diffusion
barrier in Al-LLZO, while it increases it in LGPS. The
lowering of migration barrier in Al-LLZO is in spite of
contraction of bottleneck width of Li diffusion in this
system. This finding is in line with a recent experimental
study. Analysis of EDM results shows that the lowering
(rising) in the migration barrier of Li in Al-LLZO (LGPS)
under a compressive strain is due to tendency of the system
to contract (expand) Li–O (Li–S) bond lengths in the
transition states where Li ions are at the bottlenecks of
diffusion pathways. We finally show that the result of Li
migration barrier as a function of strain in a non-doped
solid electrolyte can be used to predict the global effect
of substitution/doping on the conductivity of that system.},
cin = {IEK-1},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {113 - Methods and Concepts for Material Development
(POF3-113)},
pid = {G:(DE-HGF)POF3-113},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000537621200031},
doi = {10.1016/j.mtla.2020.100607},
url = {https://juser.fz-juelich.de/record/878028},
}