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000878129 1001_ $$0P:(DE-Juel1)174391$$aSamanta, Kartik$$b0$$eCorresponding author$$ufzj
000878129 245__ $$aCrystal Hall and crystal magneto-optical effect in thin films of SrRuO 3
000878129 260__ $$aMelville, NY$$bAmerican Inst. of Physics$$c2020
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000878129 520__ $$aMotivated by the recently observed topological Hall effect in ultra-thin films of SrRuO3 (SRO) grown on the SrTiO3 [001] substrate, we investigate the magnetic ground state and anomalous Hall response of the SRO ultra-thin films by virtue of spin density functional theory (DFT). Our findings reveal that in the monolayer limit of an SRO film, a large energy splitting of Ru-t2g states stabilizes an anti-ferromagnetic (AFM) insulating magnetic ground state. For the AFM ground state, our Berry curvature calculations predict a large anomalous Hall response upon doping. From the systematic symmetry analysis, we uncover that the large anomalous Hall effect arises due to a combination of broken time-reversal and crystal symmetries caused by the arrangement of non-magnetic atoms (Sr and O) in the SRO monolayer. We identify the emergent Hall effect as a clear manifestation of the so-called crystal Hall effect in terminology of Šmejkal et al., Crystal Hall effect in collinear antiferromagnets (2019), and demonstrate that it persists at finite frequencies, which is the manifestation of the crystal magneto-optical effect. Moreover, we find a colossal dependence of the anomalous Hall effect on the degree of crystal symmetry breaking also in ferromagnetic SRO films, which all together points to an alternative explanation of the emergence of the topological Hall effect observed in this type of systems.
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000878129 536__ $$0G:(DE-Juel1)jiff40_20190501$$aTopological transport in real materials from ab initio (jiff40_20190501)$$cjiff40_20190501$$fTopological transport in real materials from ab initio$$x2
000878129 536__ $$0G:(DE-Juel1)jiff38_20190501$$aAb initio study of novel multiferroic materials (jiff38_20190501)$$cjiff38_20190501$$fAb initio study of novel multiferroic materials$$x3
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000878129 7001_ $$0P:(DE-Juel1)130799$$aLezaic, Marjana$$b1$$ufzj
000878129 7001_ $$0P:(DE-Juel1)172668$$aMerte, Maximilian$$b2$$ufzj
000878129 7001_ $$0P:(DE-Juel1)130643$$aFreimuth, Frank$$b3
000878129 7001_ $$0P:(DE-Juel1)130548$$aBlügel, Stefan$$b4
000878129 7001_ $$0P:(DE-Juel1)130848$$aMokrousov, Yuriy$$b5$$ufzj
000878129 773__ $$0PERI:(DE-600)1476463-5$$a10.1063/5.0005017$$gVol. 127, no. 21, p. 213904 -$$n21$$p213904$$tJournal of applied physics$$v127$$x1089-7550$$y2020
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