000878196 001__ 878196
000878196 005__ 20210130005453.0
000878196 0247_ $$2doi$$a10.1063/1.5122954
000878196 0247_ $$2Handle$$a2128/25424
000878196 0247_ $$2altmetric$$aaltmetric:74735636
000878196 0247_ $$2WOS$$aWOS:000515440700001
000878196 037__ $$aFZJ-2020-02684
000878196 041__ $$aEnglish
000878196 082__ $$a530
000878196 1001_ $$00000-0002-6690-143X$$aEverhardt, Arnoud S.$$b0$$eCorresponding author
000878196 245__ $$aTemperature-independent giant dielectric response in transitional BaTiO 3 thin films
000878196 260__ $$aNew York, NY$$bAIP$$c2020
000878196 3367_ $$2DRIVER$$aarticle
000878196 3367_ $$2DataCite$$aOutput Types/Journal article
000878196 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1596462231_21261
000878196 3367_ $$2BibTeX$$aARTICLE
000878196 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000878196 3367_ $$00$$2EndNote$$aJournal Article
000878196 520__ $$aFerroelectric materials exhibit the largest dielectric permittivities and piezoelectric responses in nature, making them invaluable in applications from supercapacitors or sensors to actuators or electromechanical transducers. The origin of this behavior is their proximity to phase transitions. However, the largest possible responses are most often not utilized due to the impracticality of using temperature as a control parameter and to operate at phase transitions. This has motivated the design of solid solutions with morphotropic phase boundaries between different polar phases that are tuned by composition and that are weakly dependent on temperature. Thus far, the best piezoelectrics have been achieved in materials with intermediate (bridging or adaptive) phases. But so far, complex chemistry or an intricate microstructure has been required to achieve temperature-independent phase-transition boundaries. Here, we report such a temperature-independent bridging state in thin films of chemically simple BaTiO3. A coexistence among tetragonal, orthorhombic, and their bridging low-symmetry phases are shown to induce continuous vertical polarization rotation, which recreates a smear in-transition state and leads to a giant temperature-independent dielectric response. The current material contains a ferroelectric state that is distinct from those at morphotropic phase boundaries and cannot be considered as ferroelectric crystals. We believe that other materials can be engineered in a similar way to contain a ferroelectric state with gradual change of structure, forming a class of transitional ferroelectrics. Similar mechanisms could be utilized in other materials to design low-power ferroelectrics, piezoelectrics, dielectrics, or shape-memory alloys, as well as efficient electro- and magnetocalorics.
000878196 536__ $$0G:(DE-HGF)POF3-143$$a143 - Controlling Configuration-Based Phenomena (POF3-143)$$cPOF3-143$$fPOF III$$x0
000878196 588__ $$aDataset connected to CrossRef
000878196 7001_ $$0P:(DE-Juel1)172928$$aDenneulin, Thibaud$$b1$$ufzj
000878196 7001_ $$00000-0001-9299-058X$$aGrünebohm, Anna$$b2
000878196 7001_ $$0P:(DE-HGF)0$$aShao, Yu-Tsun$$b3
000878196 7001_ $$0P:(DE-HGF)0$$aOndrejkovic, Petr$$b4
000878196 7001_ $$0P:(DE-HGF)0$$aZhou, Silang$$b5
000878196 7001_ $$00000-0002-5229-6638$$aDomingo, Neus$$b6
000878196 7001_ $$00000-0003-0214-4828$$aCatalan, Gustau$$b7
000878196 7001_ $$00000-0002-9293-4462$$aHlinka, Jiří$$b8
000878196 7001_ $$0P:(DE-HGF)0$$aZuo, Jian-Min$$b9
000878196 7001_ $$0P:(DE-HGF)0$$aMatzen, Sylvia$$b10
000878196 7001_ $$00000-0001-8456-2286$$aNoheda, Beatriz$$b11$$eCorresponding author
000878196 773__ $$0PERI:(DE-600)2265524-4$$a10.1063/1.5122954$$gVol. 7, no. 1, p. 011402 -$$n1$$p011402 -$$tApplied physics reviews$$v7$$x1931-9401$$y2020
000878196 8564_ $$uhttps://juser.fz-juelich.de/record/878196/files/1.5122954.pdf$$yOpenAccess
000878196 8564_ $$uhttps://juser.fz-juelich.de/record/878196/files/1.5122954.pdf?subformat=pdfa$$xpdfa$$yOpenAccess
000878196 909CO $$ooai:juser.fz-juelich.de:878196$$pdnbdelivery$$pdriver$$pVDB$$popen_access$$popenaire
000878196 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)172928$$aForschungszentrum Jülich$$b1$$kFZJ
000878196 9131_ $$0G:(DE-HGF)POF3-143$$1G:(DE-HGF)POF3-140$$2G:(DE-HGF)POF3-100$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$aDE-HGF$$bEnergie$$lFuture Information Technology - Fundamentals, Novel Concepts and Energy Efficiency (FIT)$$vControlling Configuration-Based Phenomena$$x0
000878196 9141_ $$y2020
000878196 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS$$d2020-01-10
000878196 915__ $$0StatID:(DE-HGF)0160$$2StatID$$aDBCoverage$$bEssential Science Indicators$$d2020-01-10
000878196 915__ $$0LIC:(DE-HGF)CCBY4$$2HGFVOC$$aCreative Commons Attribution CC BY 4.0
000878196 915__ $$0StatID:(DE-HGF)0600$$2StatID$$aDBCoverage$$bEbsco Academic Search$$d2020-01-10
000878196 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bAPPL PHYS REV : 2018$$d2020-01-10
000878196 915__ $$0StatID:(DE-HGF)9910$$2StatID$$aIF >= 10$$bAPPL PHYS REV : 2018$$d2020-01-10
000878196 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection$$d2020-01-10
000878196 915__ $$0StatID:(DE-HGF)0110$$2StatID$$aWoS$$bScience Citation Index$$d2020-01-10
000878196 915__ $$0StatID:(DE-HGF)0111$$2StatID$$aWoS$$bScience Citation Index Expanded$$d2020-01-10
000878196 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess
000878196 915__ $$0StatID:(DE-HGF)0030$$2StatID$$aPeer Review$$bASC$$d2020-01-10
000878196 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences$$d2020-01-10
000878196 915__ $$0StatID:(DE-HGF)0430$$2StatID$$aNational-Konsortium$$d2020-01-10$$wger
000878196 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline$$d2020-01-10
000878196 915__ $$0StatID:(DE-HGF)0420$$2StatID$$aNationallizenz$$d2020-01-10$$wger
000878196 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bClarivate Analytics Master Journal List$$d2020-01-10
000878196 920__ $$lyes
000878196 9201_ $$0I:(DE-Juel1)ER-C-1-20170209$$kER-C-1$$lPhysik Nanoskaliger Systeme$$x0
000878196 980__ $$ajournal
000878196 980__ $$aVDB
000878196 980__ $$aUNRESTRICTED
000878196 980__ $$aI:(DE-Juel1)ER-C-1-20170209
000878196 9801_ $$aFullTexts