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| 100 | 1 | _ | |a Hu, Tian-Yi |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a Enhanced Energy Storage Performance of Lead-Free Capacitors in an Ultrawide Temperature Range via Engineering Paraferroelectric and Relaxor Ferroelectric Multilayer Films |
| 260 | _ | _ | |a Washington, DC |c 2020 |b Soc. |
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| 520 | _ | _ | |a Industry has been seeking a thin-film capacitor that can work at high temperature in a harsh environment, where cooling systems are not desired. Up to now, the working temperature of the thin-film capacitor is still limited up to 200 °C. Herein, we design a multilayer structure with layers of paraferroelectric (Ba0.3Sr0.7TiO3, BST) and relaxor ferroelectric (0.85BaTiO3–0.15Bi(Mg0.5Zr0.5)O3, BT–BMZ) to realize optimum properties with a flat platform of dielectric constant and high breakdown strength for excellent energy storage performance at high temperature. Through optimizing the multilayer structure, a highly stable relaxor ferroelectric state is obtained for the BST/BT–BMZ multilayer thin-film capacitor with a total thickness of 230 nm, a period number N = 8, and a layer thickness ratio of BST/BT–BMZ = 3/7. The optimized multilayer film shows significantly improved energy storage density (up to 30.64 J/cm3) and energy storage efficiency (over 70.93%) in an ultrawide temperature range from room temperature to 250 °C. Moreover, the multilayer system also exhibits excellent thermal stability in such an ultrawide temperature range with a change of 5.15 and 12.75% for the recoverable energy density and energy storage efficiency, respectively. Our results demonstrate that the designed thin-film capacitor is promising for the application in a harsh environment and open a way to tailor a thin-film capacitor toward higher working temperature with enhanced energy storage performance. |
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| 700 | 1 | _ | |a Ma, Chunrui |0 0000-0002-7824-7930 |b 1 |e Corresponding author |
| 700 | 1 | _ | |a Dai, Yanzhu |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Fan, Qiaolan |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Liu, Ming |0 P:(DE-HGF)0 |b 4 |
| 700 | 1 | _ | |a Jia, Chun-Lin |0 P:(DE-Juel1)130736 |b 5 |
| 773 | _ | _ | |a 10.1021/acsami.0c05560 |g Vol. 12, no. 23, p. 25930 - 25937 |0 PERI:(DE-600)2467494-1 |n 23 |p 25930 - 25937 |t ACS applied materials & interfaces |v 12 |y 2020 |x 1944-8252 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/878255/files/acsami.0c05560.pdf |
| 856 | 4 | _ | |y Published on 2020-05-15. Available in OpenAccess from 2021-05-15. |u https://juser.fz-juelich.de/record/878255/files/HU_TianYi.pdf |
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