001     878263
005     20210130005520.0
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100 1 _ |a Llandro, Justin
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245 _ _ |a Visualizing Magnetic Structure in 3D Nanoscale Ni–Fe Gyroid Networks
260 _ _ |a Washington, DC
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520 _ _ |a Arrays of interacting 2D nanomagnets display unprecedented electromagnetic properties via collective effects, demonstrated in artificial spin ices and magnonic crystals. Progress toward 3D magnetic metamaterials is hampered by two challenges: fabricating 3D structures near intrinsic magnetic length scales (sub-100 nm) and visualizing their magnetic configurations. Here, we fabricate and measure nanoscale magnetic gyroids, periodic chiral networks comprising nanowire-like struts forming three-connected vertices. Via block copolymer templating, we produce Ni75Fe25 single-gyroid and double-gyroid (an inversion pair of single-gyroids) nanostructures with a 42 nm unit cell and 11 nm diameter struts, comparable to the exchange length in Ni–Fe. We visualize their magnetization distributions via off-axis electron holography with nanometer spatial resolution and interpret the patterns using finite-element micromagnetic simulations. Our results suggest an intricate, frustrated remanent state which is ferromagnetic but without a unique equilibrium configuration, opening new possibilities for collective phenomena in magnetism, including 3D magnonic crystals and unconventional computing.
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536 _ _ |a 3D MAGiC - Three-dimensional magnetization textures: Discovery and control on the nanoscale (856538)
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536 _ _ |a IMAGINE - Imaging Magnetism in Nanostructures using Electron Holography (320832)
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700 1 _ |a Vyas, Kunal N.
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700 1 _ |a Cimorra, Christian
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700 1 _ |a Steiner, Ullrich
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773 _ _ |a 10.1021/acs.nanolett.0c00578
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856 4 _ |y Published on 2020-04-06. Available in OpenAccess from 2021-04-06.
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856 4 _ |y Published on 2020-04-06. Available in OpenAccess from 2021-04-06.
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