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@ARTICLE{Gliech:878265,
      author       = {Gliech, Manuel and Görlin, Mikaela and Gocyla, Martin and
                      Klingenhof, Malte and Bergmann, Arno and Selve, Sören and
                      Spöri, Camillo and Heggen, Marc and Dunin‐Borkowski,
                      Rafal E. and Suntivich, Jin and Strasser, Peter},
      title        = {{S}olute {I}ncorporation at {O}xide–{O}xide {I}nterfaces
                      {E}xplains {H}ow {T}ernary {M}ixed‐{M}etal {O}xide
                      {N}anocrystals {S}upport {E}lement‐{S}pecific
                      {A}nisotropic {G}rowth},
      journal      = {Advanced functional materials},
      volume       = {30},
      number       = {10},
      issn         = {1616-3028},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2020-02734},
      pages        = {1909054 -},
      year         = {2020},
      abstract     = {Fundamental understanding of anisotropic growth in oxide
                      nanocrystals is crucial to establish new synthesis
                      strategies and to tailor the nanoscale electronic, magnetic,
                      optical, and electrocatalytic properties of these particles.
                      While several growth investigations of metal alloy
                      nanoparticles have been reported, mechanistic studies on the
                      growth of ternary oxide materials are still missing. This
                      work constitutes the first study on the evolution of
                      anisotropic growth of manganese–cobalt oxide nanoparticles
                      by monitoring the elemental distribution and morphology
                      during the particle evolution via scanning transmission
                      electron microscopy–X‐ray spectroscopy. A new growth
                      mechanism based on a “solution‐solid‐solid” pathway
                      for mixed manganese cobalt oxides is revealed. In this
                      mechanism, the MnO seed formation occurs in the first step,
                      followed by the surface Co enrichment, which catalyzes the
                      growth along the <100> directions in all the subsequent
                      growth stages, creating rod, cross‐, and T‐shaped mixed
                      metal oxides, which preferentially expose {100} facets. It
                      is shown that the interrelation of both Mn and Co ions
                      initializes the anisotropic growth and presents the range of
                      validity of the proposed mechanism as well as the
                      shape‐determining effect based on the metal‐to‐metal
                      ratio.},
      cin          = {ER-C-1},
      ddc          = {530},
      cid          = {I:(DE-Juel1)ER-C-1-20170209},
      pnm          = {143 - Controlling Configuration-Based Phenomena (POF3-143)
                      / DFG project 257727131 - Nanoskalige Pt
                      Legierungselektrokatalysatoren mit definierter Morphologie:
                      Synthese, Electrochemische Analyse, und ex-situ/in-situ
                      Transmissionselektronenmikroskopische (TEM) Studien
                      (257727131)},
      pid          = {G:(DE-HGF)POF3-143 / G:(GEPRIS)257727131},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000507962300001},
      doi          = {10.1002/adfm.201909054},
      url          = {https://juser.fz-juelich.de/record/878265},
}