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000878280 1001_ $$0P:(DE-HGF)0$$aNerl, Hannah C.$$b0$$eCorresponding author
000878280 245__ $$aSelf‐Assembly of Atomically Thin Chiral Copper Heterostructures Templated by Black Phosphorus
000878280 260__ $$aWeinheim$$bWiley-VCH$$c2019
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000878280 520__ $$aThe fabrication of 2D systems for electronic devices is not straightforward, with top‐down low‐yield methods often employed leading to irregular nanostructures and lower quality devices. Here, a simple and reproducible method to trigger self‐assembly of arrays of high aspect‐ratio chiral copper heterostructures templated by the structural anisotropy in black phosphorus (BP) nanosheets is presented. Using quantitative atomic resolution aberration‐corrected scanning transmission electron microscopy imaging, in situ heating transmission electron microscopy and electron energy‐loss spectroscopy arrays of heterostructures forming at speeds exceeding 100 nm s−1 and displaying long‐range order over micrometers are observed. The controlled instigation of the self‐assembly of the Cu heterostructures embedded in BP is achieved using conventional electron beam lithography combined with site specific placement of Cu nanoparticles. Density functional theory calculations are used to investigate the atomic structure and suggest a metallic nature of the Cu heterostructures grown in BP. The findings of this new hybrid material with unique dimensionality, chirality, and metallic nature and its triggered self‐assembly open new and exciting opportunities for next generation, self‐assembling devices.
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000878280 7001_ $$0P:(DE-HGF)0$$aPokle, Anuj$$b1
000878280 7001_ $$0P:(DE-HGF)0$$aJones, Lewys$$b2
000878280 7001_ $$0P:(DE-HGF)0$$aMüller‐Caspary, Knut$$b3
000878280 7001_ $$0P:(DE-HGF)0$$aBos, Karel H. W.$$b4
000878280 7001_ $$0P:(DE-HGF)0$$aDowning, Clive$$b5
000878280 7001_ $$0P:(DE-HGF)0$$aMcCarthy, Eoin K.$$b6
000878280 7001_ $$0P:(DE-HGF)0$$aGauquelin, Nicolas$$b7
000878280 7001_ $$0P:(DE-HGF)0$$aRamasse, Quentin M.$$b8
000878280 7001_ $$0P:(DE-HGF)0$$aLobato, Ivan$$b9
000878280 7001_ $$0P:(DE-HGF)0$$aDaly, Dermot$$b10
000878280 7001_ $$0P:(DE-HGF)0$$aIdrobo, Juan Carlos$$b11
000878280 7001_ $$0P:(DE-HGF)0$$aVan Aert, Sandra$$b12
000878280 7001_ $$0P:(DE-HGF)0$$aVan Tendeloo, Gustaaf$$b13
000878280 7001_ $$0P:(DE-HGF)0$$aSanvito, Stefano$$b14
000878280 7001_ $$0P:(DE-HGF)0$$aColeman, Jonathan N.$$b15
000878280 7001_ $$0P:(DE-HGF)0$$aCucinotta, Clotilde S.$$b16
000878280 7001_ $$00000-0003-4814-7362$$aNicolosi, Valeria$$b17
000878280 773__ $$0PERI:(DE-600)2039420-2$$a10.1002/adfm.201903120$$gVol. 29, no. 37, p. 1903120 -$$n37$$p1903120$$tAdvanced functional materials$$v29$$x1616-3028$$y2019
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