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@ARTICLE{Nerl:878280,
      author       = {Nerl, Hannah C. and Pokle, Anuj and Jones, Lewys and
                      Müller‐Caspary, Knut and Bos, Karel H. W. and Downing,
                      Clive and McCarthy, Eoin K. and Gauquelin, Nicolas and
                      Ramasse, Quentin M. and Lobato, Ivan and Daly, Dermot and
                      Idrobo, Juan Carlos and Van Aert, Sandra and Van Tendeloo,
                      Gustaaf and Sanvito, Stefano and Coleman, Jonathan N. and
                      Cucinotta, Clotilde S. and Nicolosi, Valeria},
      title        = {{S}elf‐{A}ssembly of {A}tomically {T}hin {C}hiral
                      {C}opper {H}eterostructures {T}emplated by {B}lack
                      {P}hosphorus},
      journal      = {Advanced functional materials},
      volume       = {29},
      number       = {37},
      issn         = {1616-3028},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2020-02743},
      pages        = {1903120},
      year         = {2019},
      abstract     = {The fabrication of 2D systems for electronic devices is not
                      straightforward, with top‐down low‐yield methods often
                      employed leading to irregular nanostructures and lower
                      quality devices. Here, a simple and reproducible method to
                      trigger self‐assembly of arrays of high aspect‐ratio
                      chiral copper heterostructures templated by the structural
                      anisotropy in black phosphorus (BP) nanosheets is presented.
                      Using quantitative atomic resolution aberration‐corrected
                      scanning transmission electron microscopy imaging, in situ
                      heating transmission electron microscopy and electron
                      energy‐loss spectroscopy arrays of heterostructures
                      forming at speeds exceeding 100 nm s−1 and displaying
                      long‐range order over micrometers are observed. The
                      controlled instigation of the self‐assembly of the Cu
                      heterostructures embedded in BP is achieved using
                      conventional electron beam lithography combined with site
                      specific placement of Cu nanoparticles. Density functional
                      theory calculations are used to investigate the atomic
                      structure and suggest a metallic nature of the Cu
                      heterostructures grown in BP. The findings of this new
                      hybrid material with unique dimensionality, chirality, and
                      metallic nature and its triggered self‐assembly open new
                      and exciting opportunities for next generation,
                      self‐assembling devices.},
      cin          = {ER-C-1},
      ddc          = {530},
      cid          = {I:(DE-Juel1)ER-C-1-20170209},
      pnm          = {143 - Controlling Configuration-Based Phenomena (POF3-143)
                      / moreSTEM - Momentum-resolved Scanning Transmission
                      Electron Microscopy (VH-NG-1317)},
      pid          = {G:(DE-HGF)POF3-143 / G:(DE-HGF)VH-NG-1317},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000478478400001},
      doi          = {10.1002/adfm.201903120},
      url          = {https://juser.fz-juelich.de/record/878280},
}