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@ARTICLE{Kowalski:878372,
author = {Kowalski, Piotr},
title = {{F}ormation enthalpy of {L}n2{B}2{O}7-type
({B}={T}i,{S}n,{H}f,{Z}r) compounds},
journal = {Scripta materialia},
volume = {189},
issn = {1359-6462},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2020-02812},
pages = {7 - 10},
year = {2020},
note = {Arbeit entstand am IEK-6},
abstract = {We performed systematic ab initio calculations of the
formation enthalpies of Ln2B2O7-type (B=Ti,Sn,Hf,Zr)
compounds in pyrochlore, weberite and defect fluorite
structure. The comparison with the experimental data shows
that except the case, the defect fluorite phase is unstable
in the entire range of considered compositions and weberite
structure fits much better the measured thermochemistry
data. We found that for the Ln2Hf2O7 and Ln2Zr2O7
compositions weberite is more stable than pyrochlore for
lanthanides after Dy and Gd, respectively. This clearly
indicates the importance of the short-range ordering for
determination of stability field of pyrochlore-type
compounds.},
cin = {IEK-13 / IEK-6 / JARA-HPC},
ddc = {670},
cid = {I:(DE-Juel1)IEK-13-20190226 / I:(DE-Juel1)IEK-6-20101013 /
$I:(DE-82)080012_20140620$},
pnm = {113 - Methods and Concepts for Material Development
(POF3-113) / 161 - Nuclear Waste Management (POF3-161) /
Atomistic modeling of radionuclide-bearing materials for
safe management of high level nuclear waste.
$(jiek61_20181101)$},
pid = {G:(DE-HGF)POF3-113 / G:(DE-HGF)POF3-161 /
$G:(DE-Juel1)jiek61_20181101$},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000573816100002},
doi = {10.1016/j.scriptamat.2020.07.048},
url = {https://juser.fz-juelich.de/record/878372},
}