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@ARTICLE{Ju:878448,
author = {Ju, Min and Wu, Baohu and Sun, Shengtong and Wu, Peiyi},
title = {{R}edox‐{A}ctive {I}ron‐{C}itrate {C}omplex {R}egulated
{R}obust {C}oating‐{F}ree {H}ydrogel {M}icrofiber {N}et
with {H}igh {E}nvironmental {T}olerance and {S}ensitivity},
journal = {Advanced functional materials},
volume = {30},
number = {14},
issn = {1616-3028},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2020-02856},
pages = {1910387},
year = {2020},
abstract = {Stretchable hydrogel microfibers as a novel type of ionic
conductors are promising in gaining skin‐like sensing
applications in more diverse scenarios. However, it remains
a great challenge to fabricate coating‐free but
water‐retaining conductive hydrogel microfibers with a
good balance of spinnability and mechanical strength. Here
the old yet significant redox chemistry of Fe‐citrate
complex is employed to solve this issue in the continuous
draw‐spinning process of poly(acrylamide‐co‐sodium
acrylate) hydrogel microfibers and microfiber nets from a
water/glycerol solution. The resultant microfibers are
ionically conductive, highly stretchable, and uniform with
tunable diameters. Furthermore, the presence of
redox‐reversible Fe‐citrate complex and glycerol endows
the fibers with good anti‐freezing, water‐retaining, and
environmentally intelligent properties. Humidity and UV
light can finely mediate the stiffness of hydrogel
microfibers; conversely, the ionic conductance of
microfibers is also responsive to light, humidity, and
strain, which enables the highly sensitive perception of
environmental changes. The present draw‐spinning strategy
provides more possibilities for coating‐free conductive
hydrogel microfibers with a variety of responsive and
sensing applications.},
cin = {JCNS-FRM-II / JCNS-1 / JCNS-2 / MLZ},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-1-20110106 / I:(DE-Juel1)JCNS-2-20110106 /
I:(DE-588b)4597118-3},
pnm = {6215 - Soft Matter, Health and Life Sciences (POF3-621) /
6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)
/ 6G15 - FRM II / MLZ (POF3-6G15)},
pid = {G:(DE-HGF)POF3-6215 / G:(DE-HGF)POF3-6G4 /
G:(DE-HGF)POF3-6G15},
experiment = {EXP:(DE-MLZ)NOSPEC-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000513567300001},
doi = {10.1002/adfm.201910387},
url = {https://juser.fz-juelich.de/record/878448},
}