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000878450 245__ $$aInterfacially stable MOF nanosheet membrane with tailored nanochannels for ultrafast and thermo-responsive nanofiltration
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000878450 520__ $$aTwo-dimensional nanosheet membranes with responsive nanochannels are appealing for controlled mass transfer/separation, but limited by everchanging thicknesses arising from unstable interfaces. Herein, an interfacially stable, thermo-responsive nanosheet membrane is assembled from twin-chain stabilized metal-organic framework (MOF) nanosheets, which function via two cyclic amide-bearing polymers, thermo-responsive poly(N-vinyl caprolactam) (PVCL) for adjusting channel size, and non-responsive polyvinylpyrrolidone for supporting constant interlayer distance. Owing to the microporosity of MOF nanosheets and controllable interface wettability, the hybrid membrane demonstrates both superior separation performance and stable thermo-responsiveness. Scattering and correlation spectroscopic analyses further corroborate the respective roles of the two polymers and reveal the microenvironment changes of nanochannels are motivated by the dehydration of PVCL chains.
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000878450 7001_ $$0P:(DE-Juel1)151161$$aWu, Baohu$$b1$$ufzj
000878450 7001_ $$0P:(DE-HGF)0$$aSun, Shengtong$$b2$$eCorresponding author
000878450 7001_ $$0P:(DE-HGF)0$$aWu, Peiyi$$b3$$eCorresponding author
000878450 773__ $$0PERI:(DE-600)2442216-2$$a10.1007/s12274-020-2959-6$$p2973-2978$$tNano research$$v13$$x1998-0000$$y2020
000878450 8564_ $$uhttps://juser.fz-juelich.de/record/878450/files/Jia2020_Article_InterfaciallyStableMOFNanoshee.pdf$$yRestricted
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